[Wien] QTL-B and "Eigenvalues Below..."

Peter Blaha pblaha at theochem.tuwien.ac.at
Fri Aug 15 09:30:15 CEST 2008


Dear Stefaan,

I ran your case (exactly your input files) and had NO problems at all.
The case converges quickly and smoothly.

One possibility: You have a memory error on one of your nodes ?
Run a memory check utility and verify if the ghostbands occur always on 
the same node(s).

Peter
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.239053
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.238947
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.235192
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.235094
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.234985
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.234919
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.234905
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.234887
:ENE  : ********** TOTAL ENERGY IN Ry =      -268684.234869
homer:/area51/pblaha/lapw/tests/Ge-test-Peter> grep :dis *scf
:DIS  :  CHARGE DISTANCE       ( 0.0061557 for atom    1 spin 1) 
0.0054303
:DIS  :  CHARGE DISTANCE       ( 0.0060139 for atom    1 spin 1) 
0.0053049
:DIS  :  CHARGE DISTANCE       ( 0.0040872 for atom   10 spin 1) 
0.0019545
:DIS  :  CHARGE DISTANCE       ( 0.0027643 for atom    8 spin 1) 
0.0015330
:DIS  :  CHARGE DISTANCE       ( 0.0013487 for atom    1 spin 1) 
0.0006925
:DIS  :  CHARGE DISTANCE       ( 0.0002661 for atom   10 spin 1) 
0.0002614
:DIS  :  CHARGE DISTANCE       ( 0.0002132 for atom   10 spin 1) 
0.0002028
:DIS  :  CHARGE DISTANCE       ( 0.0001497 for atom    1 spin 1) 
0.0001233
:DIS  :  CHARGE DISTANCE       ( 0.0000427 for atom    1 spin 1) 
0.0000246



Stefaan Cottenier schrieb:
> Dear wien2k community,
> 
> I want to come back to this thread, as I did not yet succeed to identify 
> what is really going on.
> 
> To summarize the original problem: a crash in lapw2 for impurities in 
> Ge, with very large (actually ******) QTL-B warnings and (sometimes) 
> "Eigenvalues below" warnings in the preceding case.output1.
> 
> Earlier suggestions from the mailing list: keep Ge-3p in the core, take 
> larger sphere sizes for Ge. This helps in some cases, but then the 
> problem reappears in very similar cases that were before running without 
> problem.
> 
> I have now 2 test cases that show the problem, and that are as simple 
> and clean as possible. Both are a 64-atom supercell of pure bulk Ge (no 
> impurities), with the symmetry artificially lowered such that there are 
> 10 inequivalent positions. This is the diamond structure, with 4.71 au 
> between nearest neighbours. What I call case1 has Rmt=2.29 and RKM=8.01 
> for all Ge atoms (Kmax=3.5), case2 has Rmt=2.34 and RKM=8.19 (again 
> Kmax=3.5). Ge-3p states are in the core, sphere sizes are larger than in 
> my previous post, and there is now only one element involved (Ge). In 
> case1, -in1new is used, in case2 not. I discuss both these cases 
> independently. They give more or less the same errors, although some 
> details of the errors are different.
> 
> I do not succeed to reproduce this error in a smaller cell (e.g. the 
> 2-atom unit cell for the diamond structure). And it looks like the 
> problem is connected to the basis set size: often a small basis set 
> works (Kmax=2.5), but the problem appears when going to larger basis 
> sets as the Kmax=3.5 from the following two examples.
> 
> Any hints on what is going wrong?
> 
> Thanks,
> Stefaan
> 
> ----------------
> Case1
> ----------------
> This case (Rmt=2.29, RKM=8.01) was restored from a previous run, that 
> successfully finished at RKM=8.01 and without in1new. The only thing 
> that was changed for the present run, was to add -in1new 1. It crashes 
> right in the first iteration, with this error in case1.output2_4 (no 
> errors in the other 3 parts of this k-point parallel run):
> 
>    QTL-B VALUE .EQ. 1844.97972   in Band of energy   -9.34906   ATOM=    
> 5   L=  2
>     Check for ghostbands or EIGENVALUES BELOW XX messages
>     Adjust your Energy-parameters or use -in1new switch, check RMTs  !!!
> 
> There are no eigenvalues around -9.3 Ry, however, as can be seen in the 
> last iteration of the successful preceding run without -in1new:
> 
>        K=   0.12500   0.12500   0.12500            1
> :RKM  : MATRIX SIZE 8335LOs: 896  RKM= 8.01  WEIGHT= 8.00  PGR:
>        EIGENVALUES ARE:
> :EIG00001:      -1.4769260   -1.4769260   -1.4769260   -1.4769258   
> -1.4769257
> :EIG00006:      -1.4769257   -1.4767479   -1.4767478   -1.4767478   
> -1.4766416
> :EIG00011:      -1.4766416   -1.4766416   -1.4766414   -1.4766414   
> -1.4766414
> (--snip--)
> 
> This -9.3 Ry rather lies in the region of the core state energies:
> 
>         5.ATOM      Ge4                   7 CORE STATES
>        CORE-FORCE in mRy/a.u. = |F|      Fx             Fy             Fz
> :FCO005:   5.ATOM          0.004          0.000         -0.004          
> 0.000
> 
> :1S 005: 1S                -804.696867125 Ry
> :2S 005: 2S                -100.093011168 Ry
> :2PP005: 2P*                -88.951919057 Ry
> :2P 005: 2P                 -86.609329514 Ry
> :3S 005: 3S                 -11.689696508 Ry
> :3PP005: 3P*                 -8.017205664 Ry
> :3P 005: 3P                  -7.702933865 Ry
> 
> In the crashed iteration, there is an 'eigenvalues below' warning in 
> case1.output1_4 (not in the other 3 output1_* files):
> 
>       1.9669005    1.9677156    1.9730728    1.9808975    1.9813078
>       1.9815618    1.9971970    1.9973338    1.9984643
>             1 EIGENVALUES BELOW THE ENERGY  -10.00000
>        ********************************************************
> 
> The automatically produced case1.in1c looks like this (only one atom 
> shown, all other are identical to this):
> 
>  .13832   5   0      global e-param with N other choices, napw
>  0   -0.124     0.000 CONT 1
>  0   -0.421     0.000 CONT 1
>  1    0.129     0.000 CONT 1
>  2    0.106     0.000 CONT 1
>  2   -1.464     0.000 CONT 1
> 
> 
> ----------------
> Case2
> ----------------
> This case (Rmt=2.34, RKM=8.19) was started from scratch and fails in the 
> 20th iteration. In contrast to case1, no -in1new was ever used.
> 
> These are the first few eigenvalues in the last successful iteration (we 
> will need them later):
> 
>        K=   0.12500   0.12500   0.12500            1
> :RKM  : MATRIX SIZE 8335LOs: 896  RKM= 8.18  WEIGHT= 8.00  PGR:
>        EIGENVALUES ARE:
> :EIG00001:      -1.4742860   -1.4742754   -1.4742754   -1.4742486   
> -1.4742368
> :EIG00006:      -1.4742368   -1.4740887   -1.4740887   -1.4740748   
> -1.4739971
> :EIG00011:      -1.4739788   -1.4739788   -1.4739514   -1.4739514   
> -1.4739368
> :EIG00016:      -1.4737167   -1.4736918   -1.4736918   -1.4736907   
> -1.4736581
> (--snip--)
> 
> All Ge atoms show the expected linearization energies in case.scf:
> 
>           ATOMIC SPHERE DEPENDENT PARAMETERS FOR ATOM  Ge8
> :e__0009: OVERALL ENERGY PARAMETER IS    0.3000
>           OVERALL BASIS SET ON ATOM IS LAPW
> :E2_0009: E( 2)=   -1.4700   E(BOTTOM)=   -1.520   E(TOP)=   -1.420
>              APW+lo
> :E2_0009: E( 2)=    0.3000
>              LOCAL ORBITAL
> :E0_0009: E( 0)=    0.3000
>              APW+lo
> :E1_0009: E( 1)=    0.3000
>              APW+lo
> 
> And this is a part from the case2.in1c file which was used:
> 
>   0.30    4  0      (GLOBAL E-PARAMETER WITH n OTHER CHOICES, global 
> APW/LAPW)
>  2   -1.82      0.010 CONT 1
>  2    0.30      0.000 CONT 1
>  0    0.30      0.000 CONT 1
>  1    0.30      0.000 CONT 1
> 
> Now come the error messages:
> 
> In case2.output2_4 (all other 3 parts of this parallel run are OK), the 
> last lines are:
> 
>    QTL-B VALUE .EQ. **********   in Band of energy   -8.74304   ATOM=    
> 5   L=  2
>     Check for ghostbands or EIGENVALUES BELOW XX messages
>     Adjust your Energy-parameters or use -in1new switch, check RMTs  !!!
> 
> As you see from the eigenvalues printed above, there are no eigenvalues 
> in this energy range. It looks like somehow a core state is taken to be 
> a valence state...? These are the core state energies from the last 
> succesful iteration:
> 
>         2.ATOM      Ge1                   7 CORE STATES
>        CORE-FORCE in mRy/a.u. = |F|      Fx             Fy             Fz
> :FCO002:   2.ATOM          1.042          0.438          0.945          
> 0.000
> 
> :1S 002: 1S                -804.692384118 Ry
> :2S 002: 2S                -100.089338022 Ry
> :2PP002: 2P*                -88.948124153 Ry
> :2P 002: 2P                 -86.605547718 Ry
> :3S 002: 3S                 -11.686854428 Ry
> :3PP002: 3P*                 -8.014357627 Ry
> :3P 002: 3P                  -7.700089629 Ry
> 
> There were no 'Eigenvalues below' warnings in case2.output1_4, nor in 
> any of the other output1_* files:
> 
> ==> case2.output1_4 <==
>       1.9738566    1.9763199    1.9777164    1.9875908    1.9885665
>       1.9893026    1.9912437
>             0 EIGENVALUES BELOW THE ENERGY  -10.00000
>        ********************************************************
> 
> 
> 
> 
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-- 
-----------------------------------------
Peter Blaha
Inst. Materials Chemistry, TU Vienna
Getreidemarkt 9, A-1060 Vienna, Austria
Tel: +43-1-5880115671
Fax: +43-1-5880115698
email: pblaha at theochem.tuwien.ac.at
-----------------------------------------


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