[Wien] CORE electrons leak out of MT-sphere !!!!

Jinjan Ren ren at uni-muenster.de
Tue Jan 15 10:06:28 CET 2013


Dear  Laurence Marks:
              Thank you very much for your email.you are right. The structure
              should be wrong. But I don't know where is the wrong of the
              structure. The initinal structure of this C2/m (12). But in
              wien2k, there is no such space. So I convert convert C2/m to
              B2/m as  with setstru
              (http://www.cryst.ehu.es/cryst/setstru.html).  Do you think this
              is ok. The initial  and  fina structure is :









Setting Transformation
Initial structure
Initial Setting: (12)    C2/m
12
4.278 10.099 15.375 130.97 90 90
6
Au      1       -       0.000000        0.123880        0.911190
La      1       -       0.500000        0.310770        0.131320
La      2       -       0.000000        0.732630        0.672920
P       1       -       0.000000        0.449600        0.046300
P       2       -       0.500000        0.974100        0.852600
O       1       -       0.000000        0.368300        0.221000

Final structure
Final Setting: B2/m11 (12)
12 #B2/m11
10.0990 15.3750 4.2780 90.00 90.00 130.97
6
Au      1       -       0.123880        0.911190        0.000000
La      1       -       0.310770        0.131320        0.500000
La      2       -       0.732630        0.672920        0.000000
P       1       -       0.449600        0.046300        0.000000
P       2       -       0.974100        0.852600        0.500000
O       1       -       0.368300        0.221000        0.000000


Transformation matrix (P, p): b,c,a; 0,0,0
Matrix form:
(P, p) =        [     0     0     1 ] [      0]
[     1     0     0 ] [      0]
[     0     1     0 ] [      0]

Atoms Data:
AT.     WP      SS      Initial setting
Atomic Orbit    Final setting
Atomic orbit
Au1     8j x,y,z        1       (0.000000,0.123880,0.911190)
(0.000000,0.123880,0.088810)
(0.000000,0.876120,0.088810)
(0.000000,0.876120,0.911190)
(0.500000,0.623880,0.911190)
(0.500000,0.623880,0.088810)
(0.500000,0.376120,0.088810)
(0.500000,0.376120,0.911190)    (0.123880,0.911190,0.000000)
(0.123880,0.088810,0.000000)
(0.876120,0.088810,0.000000)
(0.876120,0.911190,0.000000)
(0.623880,0.911190,0.500000)
(0.623880,0.088810,0.500000)
(0.376120,0.088810,0.500000)
(0.376120,0.911190,0.500000)
La1     8j x,y,z        1       (0.500000,0.310770,0.131320)
(0.500000,0.310770,0.868680)
(0.500000,0.689230,0.868680)
(0.500000,0.689230,0.131320)
(0.000000,0.810770,0.131320)
(0.000000,0.810770,0.868680)
(0.000000,0.189230,0.868680)
(0.000000,0.189230,0.131320)    (0.310770,0.131320,0.500000)
(0.310770,0.868680,0.500000)
(0.689230,0.868680,0.500000)
(0.689230,0.131320,0.500000)
(0.810770,0.131320,0.000000)
(0.810770,0.868680,0.000000)
(0.189230,0.868680,0.000000)
(0.189230,0.131320,0.000000)
La2     8j x,y,z        1       (0.000000,0.732630,0.672920)
(0.000000,0.732630,0.327080)
(0.000000,0.267370,0.327080)
(0.000000,0.267370,0.672920)
(0.500000,0.232630,0.672920)
(0.500000,0.232630,0.327080)
(0.500000,0.767370,0.327080)
(0.500000,0.767370,0.672920)    (0.732630,0.672920,0.000000)
(0.732630,0.327080,0.000000)
(0.267370,0.327080,0.000000)
(0.267370,0.672920,0.000000)
(0.232630,0.672920,0.500000)
(0.232630,0.327080,0.500000)
(0.767370,0.327080,0.500000)
(0.767370,0.672920,0.500000)
P1      8j x,y,z        1       (0.000000,0.449600,0.046300)
(0.000000,0.449600,0.953700)
(0.000000,0.550400,0.953700)
(0.000000,0.550400,0.046300)
(0.500000,0.949600,0.046300)
(0.500000,0.949600,0.953700)
(0.500000,0.050400,0.953700)
(0.500000,0.050400,0.046300)    (0.449600,0.046300,0.000000)
(0.449600,0.953700,0.000000)
(0.550400,0.953700,0.000000)
(0.550400,0.046300,0.000000)
(0.949600,0.046300,0.500000)
(0.949600,0.953700,0.500000)
(0.050400,0.953700,0.500000)
(0.050400,0.046300,0.500000)
P2      8j x,y,z        1       (0.500000,0.974100,0.852600)
(0.500000,0.974100,0.147400)
(0.500000,0.025900,0.147400)
(0.500000,0.025900,0.852600)
(0.000000,0.474100,0.852600)
(0.000000,0.474100,0.147400)
(0.000000,0.525900,0.147400)
(0.000000,0.525900,0.852600)    (0.974100,0.852600,0.500000)
(0.974100,0.147400,0.500000)
(0.025900,0.147400,0.500000)
(0.025900,0.852600,0.500000)
(0.474100,0.852600,0.000000)
(0.474100,0.147400,0.000000)
(0.525900,0.147400,0.000000)
(0.525900,0.852600,0.000000)
O1      8j x,y,z        1       (0.000000,0.368300,0.221000)
(0.000000,0.368300,0.779000)
(0.000000,0.631700,0.779000)
(0.000000,0.631700,0.221000)
(0.500000,0.868300,0.221000)
(0.500000,0.868300,0.779000)
(0.500000,0.131700,0.779000)
(0.500000,0.131700,0.221000)    (0.368300,0.221000,0.000000)
(0.368300,0.779000,0.000000)
(0.631700,0.779000,0.000000)
(0.631700,0.221000,0.000000)
(0.868300,0.221000,0.500000)
(0.868300,0.779000,0.500000)
(0.131700,0.779000,0.500000)
(0.131700,0.221000,0.500000)


Bilbao Crystallographic Server
http://www.cryst.ehu.es         For comments, please mail to
cryst at wm.lc.ehu.es






Laurence Marks wrote on 2013-01-14:
> Your structure is wrong. RMTs of 1.1 for Au and La are unphysically
> small,
> they should be at least 2.0. And, before you ask, how it is wrong I
> do not
> know

> On Mon, Jan 14, 2013 at 11:51 AM, Jinjan Ren <ren at uni-muenster.de>
> wrote:

> > Dear all:
> >      when I do the calculation for AuLa2OP2. I always has the
> >      problem:


> > :WARNING:     0.031  Au   CORE electrons leak out of MT-sphere !!!!
> > :WARNING:     Rerun lstart with lower E-core separation energy (or
> > increase
> > sphere size)

> > :WARNING:     0.414  La   CORE electrons leak out of MT-sphere !!!!
> > :WARNING:     Rerun lstart with lower E-core separation energy (or
> > increase
> > sphere size)

> > :WARNING:     0.414  La   CORE electrons leak out of MT-sphere !!!!
> > :WARNING:     Rerun lstart with lower E-core separation energy (or
> > increase
> > sphere size)

> > :WARNING:     0.174  P    CORE electrons leak out of MT-sphere !!!!
> > :WARNING:     Rerun lstart with lower E-core separation energy (or
> > increase
> > sphere size)
> > :WARNING:     ORBITAL:  2P*    -9.172    -9.141
> > :WARNING:     ORBITAL:  2P     -9.104    -9.074

> > :WARNING:     0.174  P    CORE electrons leak out of MT-sphere !!!!
> > :WARNING:     Rerun lstart with lower E-core separation energy (or
> > increase
> > sphere size)
> > :WARNING:     ORBITAL:  2P*    -9.172    -9.141
> > :WARNING:     ORBITAL:  2P     -9.104    -9.074
> > LSTART ENDS
> > 0.952u 0.052s 0:00.98 102.0%    0+0k 0+2640io 0pf

> > I have tried the value of Ry from -6 to -12, when the values are
> > from -6 to
> > -10  above problems always there. But when I set the value to be
> > more than
> > -10
> > another problem is:

> > forrtl: severe (24): end-of-file during read, unit -4, file stdin
> > Image              PC                Routine            Line
> > Source
> > lstart             00000000004AB271  Unknown               Unknown
> > Unknown
> > lstart             00000000004AA245  Unknown               Unknown
> > Unknown
> > lstart             000000000045AABA  Unknown               Unknown
> > Unknown
> > lstart             0000000000424205  Unknown               Unknown
> > Unknown
> > lstart             00000000004239FA  Unknown               Unknown
> > Unknown
> > lstart             0000000000440C81  Unknown               Unknown
> > Unknown
> > lstart             000000000043E9B0  Unknown               Unknown
> > Unknown
> > lstart             000000000040F23B  MAIN__                     63
> >  lstart.f
> > lstart             000000000040363C  Unknown               Unknown
> > Unknown
> > libc.so.6          00002AE235EDE586  Unknown               Unknown
> > Unknown
> > lstart             0000000000403539  Unknown               Unknown
> > Unknown
> > 0.000u 0.000s 0:00.00 0.0%      0+0k 0+0io 0pf+0w
> > error: command   /opt/w2k/lstart lstart.def   failed


> > The distance between the nuclei are:

> >   please specify nn-bondlength factor: (usually=2)
> >  DSTMAX:   20.0000000000000
> >  gamma not equal 90

> >     ATOM  1  Au         ATOM  2  La
> >  RMT(  1)=1.10000 AND RMT(  2)=1.10000
> >  SUMS TO 2.20000  LT.  NN-DIST= 2.25851

> >     ATOM  2  La         ATOM  1  Au
> >  RMT(  2)=1.10000 AND RMT(  1)=1.10000
> >  SUMS TO 2.20000  LT.  NN-DIST= 2.25851

> >     ATOM  3  La         ATOM  6  O
> >  RMT(  3)=1.10000 AND RMT(  6)=2.10000
> >  SUMS TO 3.20000  LT.  NN-DIST= 4.58198

> >     ATOM  4  P          ATOM  5  P
> >  RMT(  4)=1.10000 AND RMT(  5)=1.10000
> >  SUMS TO 2.20000  LT.  NN-DIST= 2.26712

> >     ATOM  5  P          ATOM  4  P
> >  RMT(  5)=1.10000 AND RMT(  4)=1.10000
> >  SUMS TO 2.20000  LT.  NN-DIST= 2.26712

> >     ATOM  6  O          ATOM  2  La
> >  RMT(  6)=2.10000 AND RMT(  2)=1.10000
> >  SUMS TO 3.20000  LT.  NN-DIST= 4.53674
> > NN ENDS
> > 0.020u 0.004s 0:00.00 0.0%      0+0k 0+176io 0pf+0w







> > _______________________________________________
> > Wien mailing list
> > Wien at zeus.theochem.tuwien.ac.at
> > http://zeus.theochem.tuwien.ac.at/mailman/listinfo/wien




> --
> Professor Laurence Marks
> Department of Materials Science and Engineering
> Northwestern University
> www.numis.northwestern.edu 1-847-491-3996
> "Research is to see what everybody else has seen, and to think what
> nobody
> else has thought"
> Albert Szent-Gyorgi


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