[Wien] First time doing volume optimization

Peter Blaha pblaha at theochem.tuwien.ac.at
Fri May 17 15:56:16 CEST 2013


You said: I want to do a volume optimization and you started with a 
"cubic" structure.

Thus you should NOT click on optimization V+c/a  !!!  This requires a 
tetragonal setup (which you probably don't have).

Just do a VOLUME optimization alone. You have to specify which volume 
changes you want to do,... (see UG quick start).

On 05/17/2013 02:55 PM, Oleg Rubel wrote:
> Dear Wasim,
>
> for the peroskite structure, make sure that you run 'mini' for each and every combination of volume & c/a (non-centrosymmetric structure) with tight force convergence (lower than 1 mRy/Bohr) in order to ensure smooth energy profile.
>
> The number of k-point is reduced due to the symmetry of the cubic structure. Your non-centrosymmetric case will have a larger # of k-point for the same mesh.
>
> When you try out all possibilities (V & c/a), I would take the lowest symmetry structure as a reference for initialization. This will ensure that the # of k-point and symmetry operations do NOT change through the calculation resulting in a consistent energy profile.
>
> I cannot comment on questions (1) and (2), since we still do it in an old fashion (choose particular V and vary c/a at V=const). We should try a newer approach, probably.
>
>
> Regards
> Oleg
>
>>>> On 5/17/2013 at 2:57 AM, in message
> <CAGfip2XGtK7XaCj99EqUqeETk9yOrDMkHv2HgMfbfMDjQG4wPw at mail.gmail.com>, wasim
> raja Mondal <wasimr.mondal at gmail.com> wrote:
>> Dear wien2k experts
>>
>>       I am doing volume optimization of one peroskite structure and want to
>> calculate the optimized lattice parameter. It is a perfect cubic structure
>> and experimental lattice parameter is 4.0029 angstrom. After initilizing
>> all the step, I have clicked on optimize (v,c/a) and it wanted input
>> parameter for a:b:c ratio. For that I have given as -2, -2, -2 and run the
>> calculation. It has run with no error and came out successfully. According
>> to the manual, a file case.outputeos should have been created . But I have
>> not found. I have the following question:
>>
>>
>> (1) what should be the generally  appropriate value to put for the a:b:c
>> for the volume optimize?
>>
>> (2)After run, where can I find my optimize lattice parameter value ?
>>
>> (3) In the prepare input file for the k-point I have given 2744 number of
>> k-points. I wanted k-mesh as 14*14*14. But   in the created
>> "cubic_phase_vol__-2.0.scf" it is showing number of k-points is 84. Why?
>>
>>
>> I am giving the day file below so that some body can comment it is
>> correctly done or not?
>> My day file is following:
>>
>> Calculating cubic_phase in /home/raja/BaRuO3/cubic_phase
>> on viper5 with PID 30191
>> using WIEN2k_12.1 (Release 22/7/2012) in /home/raja/wien2k_installation
>>
>>
>>      start 	(Fri May 17 17:07:21 IST 2013) with lapw0 (40/99 to go)
>>
>>      cycle 1 	(Fri May 17 17:07:21 IST 2013) 	(40/99 to go)
>>
>>>    lapw0 	(17:07:21) 2.7u 0.0s 0:02.80 99.6% 0+0k 0+672io 0pf+0w
>>>    lapw1     	(17:07:23)  _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>> 13.0u 0.2s 0:13.38 99.7% 0+0k 0+35872io 0pf+0w
>>>    lapw2     	(17:07:37) 3.6u 0.1s 0:03.76 99.7% 0+0k 0+712io 0pf+0w
>>>    lcore	(17:07:41) 0.0u 0.0s 0:00.03 66.6% 0+0k 0+352io 0pf+0w
>>>    mixer	(17:07:41) 0.0u 0.0s 0:00.04 75.0% 0+0k 0+984io 0pf+0w
>> :ENERGY convergence:  0 0.0001 0
>> :CHARGE convergence:  0 0.0000 0
>> ec cc and fc_conv 0 1 1
>>
>>      cycle 2 	(Fri May 17 17:07:41 IST 2013) 	(39/98 to go)
>>
>>>    lapw0 	(17:07:41) 2.8u 0.0s 0:02.90 99.6% 0+0k 0+672io 0pf+0w
>>>    lapw1     	(17:07:44)  _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>> 13.0u 0.3s 0:13.44 99.7% 0+0k 0+35872io 0pf+0w
>>>    lapw2     	(17:07:57) 3.6u 0.1s 0:03.77 99.7% 0+0k 0+712io 0pf+0w
>>>    lcore	(17:08:01) 0.0u 0.0s 0:00.03 66.6% 0+0k 0+352io 0pf+0w
>>>    mixer	(17:08:01) 0.0u 0.0s 0:00.05 100.0% 0+0k 0+976io 0pf+0w
>> :ENERGY convergence:  0 0.0001 0
>> :CHARGE convergence:  0 0.0000 0
>> ec cc and fc_conv 0 1 1
>>
>>      cycle 3 	(Fri May 17 17:08:01 IST 2013) 	(38/97 to go)
>>
>>>    lapw0 	(17:08:01) 2.9u 0.0s 0:02.94 99.6% 0+0k 0+672io 0pf+0w
>>>    lapw1     	(17:08:04)  _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>>   _nb in dscgst.F         640         128
>> 13.1u 0.3s 0:13.47 99.7% 0+0k 0+35864io 0pf+0w
>>>    lapw2     	(17:08:18) 3.6u 0.1s 0:03.77 99.7% 0+0k 0+712io 0pf+0w
>>>    lcore	(17:08:22) 0.0u 0.0s 0:00.03 66.6% 0+0k 0+352io 0pf+0w
>>>    mixer	(17:08:22) 0.0u 0.0s 0:00.07 71.4% 0+0k 0+992io 0pf+0w
>> :ENERGY convergence:  1 0.0001 .0000000650000000
>> :CHARGE convergence:  0 0.0000 .0001101
>> ec cc and fc_conv 1 1 1
>>
>>>    stop
>>
>>
>> Regards
>> wasim
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-- 

                                       P.Blaha
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Peter BLAHA, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna
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