[Wien] Nuclear charge shows as lowered with core hole (:NEC lines)

Peter Blaha pblaha at theochem.tuwien.ac.at
Mon Mar 23 16:06:12 CET 2015


This is ok. What is printed is the sum of nuclear charges - background, 
so that you can more easily compare this number with that of the 
electronic charge (where there is a tiny core-leakage too).


On 03/23/2015 04:03 PM, David Olmsted wrote:
> Hi,
>   I am using WIEN2k_14.2 (Release 15/10/2014).  I am doing a calculation with
> a half core-hole, offset by background charge, in order to model XPS.
>
> The :NEC lines in case.scf and case.scfm show:
>   Al2O3_super.scf::NEC01: NUCLEAR AND ELECTRONIC CHARGE    299.50000
> 299.49192
>   Al2O3_super.scf::NEC02: NUCLEAR AND ELECTRONIC CHARGE    299.50000
>   299.50000
>   Al2O3_super.scf::NEC03: NUCLEAR AND ELECTRONIC CHARGE    299.50000
> 299.50000
> But the nuclear charge should be 300.  (No changes in the case.struct file
> for the half core-hole.)
>
> Is this an error on my part, or an error in the calculation, or just
> something in the reporting?  (I was unable to find anything on this in the
> mail archive.)
>
> case.stuct, case.inc and case.inm follow.
>
> Thanks,
>   David
>
>   David Olmsted
>   Assistant Research Engineer
>   Materials Science and Engineering
>   210 Hearst Memorial Mining Building
>   University of California
>   Berkeley, CA 94720-1760
>
>   ------------ case.struct -----------------
>
> Al2O3_gga
>
>   H   LATTICE,NONEQUIV.ATOMS: 18 143
> P3
>
>               RELA
>
>     9.130402  9.130402 24.917749 90.000000
> 90.000000120.000000
>   ATOM  -1: X=0.00000000 Y=0.00000000 Z=0.00000000
>             MULT= 1          ISPLIT= 4
>   Al1        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM  -2: X=0.33333333 Y=0.66666667 Z=0.66666667
>             MULT= 1          ISPLIT= 4
>   Al2        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM  -3: X=0.66666667 Y=0.33333333 Z=0.33333333
>             MULT= 1          ISPLIT= 4
>   Al3        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM  -4: X=0.33333333 Y=0.66666667 Z=0.37066957
>             MULT= 1          ISPLIT= 4
>   Al4        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM  -5: X=0.33333333 Y=0.66666667 Z=0.16666667
>             MULT= 1          ISPLIT= 4
>   Al5        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM  -6: X=0.66666667 Y=0.33333333 Z=0.83333333
>             MULT= 1          ISPLIT= 4
>   Al6        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM  -7: X=0.33333333 Y=0.66666667 Z=0.87066957
>             MULT= 1          ISPLIT= 4
>   Al7        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM  -8: X=0.66666667 Y=0.33333333 Z=0.03733623
>             MULT= 1          ISPLIT= 4
>   Al8        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM  -9: X=0.66666667 Y=0.33333333 Z=0.53733623
>             MULT= 1          ISPLIT= 4
>   Al9        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -10: X=0.97274955 Y=0.33333333 Z=0.43533478
>             MULT= 3          ISPLIT= 8
>        -10: X=0.66666667 Y=0.63941622 Z=0.43533478
>        -10: X=0.36058378 Y=0.02725045 Z=0.43533478
>   O 1        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 8.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -11: X=0.02725045 Y=0.66666667 Z=0.26866812
>             MULT= 3          ISPLIT= 8
>        -11: X=0.33333333 Y=0.36058378 Z=0.26866812
>        -11: X=0.63941622 Y=0.97274955 Z=0.26866812
>   O 2        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 8.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -12: X=0.30608288 Y=0.00000000 Z=0.10200145
>             MULT= 3          ISPLIT= 8
>        -12: X=0.00000000 Y=0.30608288 Z=0.10200145
>        -12: X=0.69391712 Y=0.69391712 Z=0.10200145
>   O 3        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 8.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -13: X=0.36058379 Y=0.33333333 Z=0.93533478
>             MULT= 3          ISPLIT= 8
>        -13: X=0.66666667 Y=0.02725046 Z=0.93533478
>        -13: X=0.97274954 Y=0.63941621 Z=0.93533478
>   O 4        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 8.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -14: X=0.63941621 Y=0.66666667 Z=0.76866812
>             MULT= 3          ISPLIT= 8
>        -14: X=0.33333333 Y=0.97274954 Z=0.76866812
>        -14: X=0.02725046 Y=0.36058379 Z=0.76866812
>   O 5        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 8.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -15: X=0.69391712 Y=0.00000000 Z=0.60200145
>             MULT= 3          ISPLIT= 8
>        -15: X=0.00000000 Y=0.69391712 Z=0.60200145
>        -15: X=0.30608288 Y=0.30608288 Z=0.60200145
>   O 6        NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 8.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -16: X=0.00000000 Y=0.00000000 Z=0.70400290
>             MULT= 1          ISPLIT= 4
>   Al10       NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -17: X=0.00000000 Y=0.00000000 Z=0.50000000
>             MULT= 1          ISPLIT= 4
>   Al11       NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>   ATOM -18: X=0.00000000 Y=0.00000000 Z=0.20400290
>             MULT= 1          ISPLIT= 4
>   Al12       NPT=  781  R0=0.00010000 RMT=    1.7100   Z:
> 13.0
>   LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>                        0.0000000 1.0000000 0.0000000
>                        0.0000000 0.0000000 1.0000000
>      3      NUMBER OF SYMMETRY OPERATIONS
>   1 0 0 0.00000000
>   0 1 0 0.00000000
>   0 0 1 0.00000000
>          1
>   0-1 0 0.00000000
>   1-1 0 0.00000000
>   0 0 1 0.00000000
>          2
>   -1 1 0 0.00000000
>   -1 0 0 0.00000000
>   0 0 1 0.00000000
>          3
>   ------------------------------ case.inm ---------------------------------
>   MSR1  -0.5   YES  (BROYD/PRATT, BG charge (-1 for core hole), norm)
>   0.20            mixing FACTOR for BROYD/PRATT scheme
>   1.00  1.00      PW and CLM-scaling factors
>   9999  8        idum, HISTORY
>   ------------------------------ case.inc
> ------------------------------------
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,1.5             ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   1 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   1 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   1 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   1 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   1 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   1 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   4 0.00  0  NUMBER OF ORBITALS (EXCLUDING SPIN), SHIFT, IPRINT
>   1,-1,2               ( N,KAPPA,OCCUP)
>   2,-1,2               ( N,KAPPA,OCCUP)
>   2, 1,2               ( N,KAPPA,OCCUP)
>   2,-2,4               ( N,KAPPA,OCCUP)
>   0
>   ----------------------------------
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-- 

                                       P.Blaha
--------------------------------------------------------------------------
Peter BLAHA, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna
Phone: +43-1-58801-165300             FAX: +43-1-58801-165982
Email: blaha at theochem.tuwien.ac.at    WIEN2k: http://www.wien2k.at
WWW:   http://www.imc.tuwien.ac.at/staff/tc_group_e.php
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