[Wien] Optic program error for XMCD calculation of Fe3O4

Peter Blaha pblaha at theochem.tuwien.ac.at
Wed Jul 4 11:02:09 CEST 2018


I could finally make the XMCD option working again. Several small errors 
were fixed in a preliminary way, because of a partial (incomplete) HELO 
implementation. HELOs are still not supported for XMCD. Cells with more 
than one atom should work now (I guess they never worked ??).

However, I have not verified the results against previous versions (for 
bcc Fe), nor made other cross checks (eg. run bcc Fe in simple cubic 
structure with 2 atoms, ...). So please check.

The modifications are too big to send them here.

However, I'm ready now with WIEN2k_18, where these fixes will be 
included. The new release should come today/tomorrow, unless I find some 
more problems.

Peter Blaha

On 06/27/2018 02:40 PM, Jose Maria Castillo wrote:
> Yes, I tried with bcc-Fe and I didn't have any problem.
> 
> Best regards,
> 
> José María Castillo Robles
> El mié., 27 de jun. de 2018 a la(s) 03:34, Peter Blaha
> (pblaha at theochem.tuwien.ac.at) escribió:
>>
>> Did you try bccFe ?? This runs for me (and I would like to get a hint if
>> the problem comes from more atoms/cell or if your optics is not updated
>> properly)
>>
>> On 06/27/2018 08:07 AM, Jose Maria Castillo wrote:
>>> Dear Prof. Blaha,
>>>
>>> Thank you for your answer.  Yes, I used the patch that is in the following post:
>>>
>>> https://www.mail-archive.com/wien@zeus.theochem.tuwien.ac.at/msg17555.html
>>>
>>> but I got the error that I mentioned.
>>>
>>> Best regards,
>>>
>>> José María Castillo Robles
>>>
>>> El mié., 27 de jun. de 2018 a la(s) 00:26, Peter Blaha
>>> (pblaha at theochem.tuwien.ac.at) escribió:
>>>>
>>>> Did you search the mailinglist for recent threads about xmcd ?
>>>>
>>>> There was a patch for a severe bug mentioned just a few weeks ago.
>>>>
>>>> Regards
>>>>
>>>> Am 27.06.2018 um 07:11 schrieb Jose Maria Castillo:
>>>>> Dear Prof. Blaha and Wien2k users,
>>>>>
>>>>> I am using WIEN2k version WIEN2k_17.1 for calculating XMCD spectra of
>>>>> Fe3O4 at the L23 edge for Fe.  First, I did a spin polarized
>>>>> calculation using:
>>>>>
>>>>> init_lapw (using default settings)
>>>>> runsp_lapw -ec 0.0001
>>>>>
>>>>> and then a calculation including spin orbit coupling. I ran the
>>>>> following commands:
>>>>>
>>>>> initso_lapw (using default settings)
>>>>> rm *.broyd*
>>>>> runsp_lapw -so -ec 0.0001
>>>>>
>>>>> and I don't get any errors in the calculations. In both cases, the
>>>>> Brillouin zone was sampled with 1000 k-points.
>>>>>
>>>>> After this, I ran the commands that are mentioned in the usersguide
>>>>> (section 8.17 "OPTIC calculating optical properties") :
>>>>>
>>>>> 1. cp Fe3O4.struct Fe3O4.ksym
>>>>> 2. x kgen -so -fbz
>>>>> 3. change TOT to FERMI in Fe3O4.in2c and Fe3O4.in2
>>>>> 4. put TETRA with value 101 in Fe3O4.in2c and Fe3O4.in2
>>>>> 5. set IPRINT=1 in Fe3O4.inc
>>>>> 6. rm *broyd*
>>>>> 7. x lapw1 -up
>>>>> 8. x lapw1 -dn
>>>>> 9. x lapwso -up
>>>>> 10. x lapw2 -fermi -up
>>>>> 11. x lapw2 -fermi -dn
>>>>> 12. x lcore -up
>>>>> 13. x lcore -dn
>>>>> 14. x optic -so -up
>>>>>
>>>>> Before optic program, it ran without errors, but after running optic
>>>>> program it crashes with the following error:
>>>>>
>>>>>
>>>>> user at machine:~/Fe3O4$ x optic -so -up
>>>>>     emin,emax,nbvalmax  -5.00000000000000        3.00000000000000             9999
>>>>>     XMCD selected for atom           2 L23
>>>>>     LSO=  T
>>>>> forrtl: severe (64): input conversion error, unit 18, file
>>>>> /home/user/Fe3O4/Fe3O4.vspup
>>>>> Image              PC                Routine            Line
>>>>> Source
>>>>> opticc             0000000000436D53  Unknown               Unknown  Unknown
>>>>> opticc             000000000045C00A  Unknown               Unknown  Unknown
>>>>> opticc             0000000000403709  atpar_                     62  atpar_op.f
>>>>> opticc             0000000000429D22  cor_mat_                  345
>>>>> sph-UPcor_tmp.f
>>>>> opticc             00000000004112F1  MAIN__                    460  opmain.f
>>>>> opticc             0000000000402BEE  Unknown               Unknown  Unknown
>>>>> libc-2.23.so       00002AE5A5E03830  __libc_start_main     Unknown  Unknown
>>>>> opticc             0000000000402AE9  Unknown               Unknown  Unknown
>>>>> 0.0u 0.0s 0:00.01 100.0% 0+0k 0+72io 0pf+0w
>>>>> error: command   /home/user/WIEN2k_ifort/opticc upoptic.def   failed
>>>>>
>>>>> In order to discard a problem with the structure, I tried to do the
>>>>> XMCD calculation for two different solids (Fe3O4 and CeFe2)
>>>>> and I got the same error. It looks like the format of Fe3O4.vspup is
>>>>> not compatible with optic program.
>>>>>
>>>>> I would like to ask for your help. I send you the input files for the
>>>>> optic program, the output, as well as the error files.
>>>>>
>>>>> Thanks in advance for your help.
>>>>>
>>>>> Best regards!
>>>>> José María Castillo Robles
>>>>> -------------------------Inputs--------------------------------------------
>>>>> Fe3O4.inop
>>>>> 99999 1       number of k-points, first k-point
>>>>> -5.0 3.0 9999 Emin, Emax for matrix elements, NBvalMAX
>>>>> XMCD 1 L23    xmcd  atom_num edge
>>>>> 2             number of choices (columns in *outmat): 2: hex or tetrag. case
>>>>> 1             Re xx
>>>>> 3             Re zz
>>>>> OFF           ON/OFF   writes MME to unit 4
>>>>> -----------------------------------------------------------------------------------------------
>>>>> Fe3O4.inc
>>>>>     1 0.00  1  NUMBER OF ORBITALS (EXCLUDING SPIN)
>>>>> 1,-1,2               ( N,KAPPA,OCCUP)
>>>>>     5 0.00  1  NUMBER OF ORBITALS (EXCLUDING SPIN)
>>>>> 1,-1,2               ( N,KAPPA,OCCUP)
>>>>> 2,-1,2               ( N,KAPPA,OCCUP)
>>>>> 2, 1,2               ( N,KAPPA,OCCUP)
>>>>> 2,-2,4               ( N,KAPPA,OCCUP)
>>>>> 3,-1,2               ( N,KAPPA,OCCUP)
>>>>>     5 0.00  1  NUMBER OF ORBITALS (EXCLUDING SPIN)
>>>>> 1,-1,2               ( N,KAPPA,OCCUP)
>>>>> 2,-1,2               ( N,KAPPA,OCCUP)
>>>>> 2, 1,2               ( N,KAPPA,OCCUP)
>>>>> 2,-2,4               ( N,KAPPA,OCCUP)
>>>>> 3,-1,2               ( N,KAPPA,OCCUP)
>>>>>     0
>>>>> -------------------------------------------------------------------------------------------------
>>>>> Fe3O4.in2c and Fe3O4.in2
>>>>> FERMI           (TOT,FOR,QTL,EFG,FERMI)
>>>>>       -12.0   132.0   0.50 0.05  1   EMIN, NE, ESEPERMIN, ESEPER0, iqtls
>>>>> TETRA    101        (GAUSS,ROOT,TEMP,TETRA,ALL      eval)
>>>>>      0 0  1 1 -1 1  2 0  2 2 -2 2  3 1 -3 1  3 3 -3 3  4 0  4 2 -4 2  4 4
>>>>> -4 4  5 1 -5 1  5 3 -5 3  5 5 -5 5  6 0  6 2 -6 2  6 4 -6 4  6 6 -6 6
>>>>>      0 0  2 0  2 2 -2 2  4 0  4 2 -4 2  4 4 -4 4  6 0  6 2 -6 2  6 4 -6 4  6 6 -6 6
>>>>>      0 0  2 0 -3 2  4 0  4 4 -5 2  6 0  6 4
>>>>>     12.00          GMAX
>>>>> NOFILE        FILE/NOFILE  write recprlist
>>>>> ----------------------------------------------------------------------------------------------------
>>>>> Fe3O4.struct
>>>>> Fe3o4                                    s-o calc. M||  0.00  0.00  1.00
>>>>> F                            3 227_
>>>>>                 RELA
>>>>>     15.864257 15.864257 15.864257 90.000000 90.000000 90.000000
>>>>> ATOM  -1: X=0.24450000 Y=0.24450000 Z=0.24450000
>>>>>              MULT= 8          ISPLIT= 8
>>>>>          -1: X=0.75550000 Y=0.75550000 Z=0.75550000
>>>>>          -1: X=0.75550000 Y=0.49450000 Z=0.49450000
>>>>>          -1: X=0.24450000 Y=0.00550000 Z=0.00550000
>>>>>          -1: X=0.00550000 Y=0.00550000 Z=0.24450000
>>>>>          -1: X=0.49450000 Y=0.49450000 Z=0.75550000
>>>>>          -1: X=0.49450000 Y=0.75550000 Z=0.49450000
>>>>>          -1: X=0.00550000 Y=0.24450000 Z=0.00550000
>>>>> O 1        NPT=  781  R0=.000100000 RMT=   1.65000   Z:   8.00000
>>>>> LOCAL ROT MATRIX:    0.0000000-0.7071068-0.7071068
>>>>>                         0.0000000-0.7071068 0.7071068
>>>>>                        -1.0000000 0.0000000 0.0000000
>>>>> ATOM  -2: X=0.00000000 Y=0.00000000 Z=0.00000000
>>>>>              MULT= 4          ISPLIT= 8
>>>>>          -2: X=0.00000000 Y=0.25000000 Z=0.25000000
>>>>>          -2: X=0.25000000 Y=0.25000000 Z=0.00000000
>>>>>          -2: X=0.25000000 Y=0.00000000 Z=0.25000000
>>>>> Fe1        NPT=  781  R0=.000050000 RMT=   1.92000   Z:  26.00000
>>>>> LOCAL ROT MATRIX:    0.0000000-0.7071068-0.7071068
>>>>>                         0.0000000-0.7071068 0.7071068
>>>>>                        -1.0000000 0.0000000 0.0000000
>>>>> ATOM  -3: X=0.37500000 Y=0.37500000 Z=0.37500000
>>>>>              MULT= 2          ISPLIT=-2
>>>>>          -3: X=0.62500000 Y=0.62500000 Z=0.62500000
>>>>> Fe2        NPT=  781  R0=.000050000 RMT=   1.92000   Z:  26.00000
>>>>> LOCAL ROT MATRIX:    1.0000000 0.0000000 0.0000000
>>>>>                         0.0000000 1.0000000 0.0000000
>>>>>                         0.0000000 0.0000000 1.0000000
>>>>>      16      NUMBER OF SYMMETRY OPERATIONS
>>>>> -1 0 0 0.00000000
>>>>>     0-1 0 0.00000000
>>>>>     0 0-1 0.00000000
>>>>>           1   A   1 so. oper.  type  orig. index
>>>>>     1 0 0 0.00000000
>>>>>     0 1 0 0.00000000
>>>>>     0 0 1 0.00000000
>>>>>           2   A  12
>>>>>     0-1 0 0.25000000
>>>>>     1 0 0 0.00000000
>>>>>     0 0-1 0.25000000
>>>>>           3   A  15
>>>>>     1 0 0 0.75000000
>>>>>     0 1 0 0.75000000
>>>>>     0 0-1 0.00000000
>>>>>           4   A  18
>>>>>     0 1 0 0.00000000
>>>>> -1 0 0 0.25000000
>>>>>     0 0-1 0.25000000
>>>>>           5   A  22
>>>>> -1 0 0 0.25000000
>>>>>     0-1 0 0.25000000
>>>>>     0 0 1 0.00000000
>>>>>           6   A  33
>>>>>     0 1 0 0.75000000
>>>>> -1 0 0 0.00000000
>>>>>     0 0 1 0.75000000
>>>>>           7   A  36
>>>>>     0-1 0 0.00000000
>>>>>     1 0 0 0.75000000
>>>>>     0 0 1 0.75000000
>>>>>           8   A  45
>>>>>     0-1 0 0.00000000
>>>>> -1 0 0 0.00000000
>>>>>     0 0-1 0.00000000
>>>>>           9   B   3
>>>>>     0 1 0 0.00000000
>>>>>     1 0 0 0.00000000
>>>>>     0 0 1 0.00000000
>>>>>          10   B  10
>>>>> -1 0 0 0.00000000
>>>>>     0 1 0 0.75000000
>>>>>     0 0 1 0.75000000
>>>>>          11   B  13
>>>>>     1 0 0 0.00000000
>>>>>     0-1 0 0.25000000
>>>>>     0 0-1 0.25000000
>>>>>          12   B  14
>>>>> -1 0 0 0.25000000
>>>>>     0 1 0 0.00000000
>>>>>     0 0-1 0.25000000
>>>>>          13   B  19
>>>>>     0 1 0 0.75000000
>>>>>     1 0 0 0.75000000
>>>>>     0 0-1 0.00000000
>>>>>          14   B  28
>>>>>     1 0 0 0.75000000
>>>>>     0-1 0 0.00000000
>>>>>     0 0 1 0.75000000
>>>>>          15   B  32
>>>>>     0-1 0 0.25000000
>>>>> -1 0 0 0.25000000
>>>>>     0 0 1 0.00000000
>>>>>          16   B  43
>>>>> --------------------Output------------------------------------------------------------------------------
>>>>> Fe3O4.outputopup
>>>>>
>>>>>                                  --------------------------------------------------
>>>>>                                     S T R U C T U R A L   I N F O R M A T I O N
>>>>>                                  --------------------------------------------------
>>>>>
>>>>>
>>>>>       SUBSTANCE                    = Fe3o4
>>>>>        s-o calc. M||  0.00  0.00  1.00
>>>>>
>>>>>       LATTICE                      = F
>>>>>       LATTICE CONSTANTS ARE        =   15.8642570  15.8642570  15.8642570
>>>>>       NUMBER OF ATOMS IN UNITCELL  =   3
>>>>>       MODE OF CALCULATION IS       = RELA
>>>>>       MODUSALL
>>>>>       spin-polarized calculation
>>>>>       spin-orbit coupling included
>>>>>     read inso:
>>>>>     theta=  0.000000000000000E+000
>>>>>     phi=  0.000000000000000E+000
>>>>>     call trans..
>>>>>     Transf. matrix:  -1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  -1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>      -1.00000000000000
>>>>>     operation           1
>>>>>     det:   1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:   1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000   1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>       1.00000000000000
>>>>>     operation           2
>>>>>     det:   1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  0.000000000000000E+000   1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  -1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>      -1.00000000000000
>>>>>     operation           3
>>>>>     det:   1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:   1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000   1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>      -1.00000000000000
>>>>>     operation           4
>>>>>     det:   1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  0.000000000000000E+000  -1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:   1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>      -1.00000000000000
>>>>>     operation           5
>>>>>     det:   1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  -1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  -1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>       1.00000000000000
>>>>>     operation           6
>>>>>     det:   1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  0.000000000000000E+000  -1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:   1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>       1.00000000000000
>>>>>     operation           7
>>>>>     det:   1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  0.000000000000000E+000   1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  -1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>       1.00000000000000
>>>>>     operation           8
>>>>>     det:   1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  0.000000000000000E+000  -1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  -1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>      -1.00000000000000
>>>>>     operation           9
>>>>>     det:  -1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  0.000000000000000E+000   1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:   1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>       1.00000000000000
>>>>>     operation          10
>>>>>     det:  -1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  -1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000   1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>       1.00000000000000
>>>>>     operation          11
>>>>>     det:  -1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:   1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  -1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>      -1.00000000000000
>>>>>     operation          12
>>>>>     det:  -1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  -1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000   1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>      -1.00000000000000
>>>>>     operation          13
>>>>>     det:  -1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  0.000000000000000E+000   1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:   1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>      -1.00000000000000
>>>>>     operation          14
>>>>>     det:  -1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:   1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  -1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>       1.00000000000000
>>>>>     operation          15
>>>>>     det:  -1.00000000000000
>>>>>     call trans..
>>>>>     Transf. matrix:  0.000000000000000E+000  -1.00000000000000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  -1.00000000000000       0.000000000000000E+000
>>>>>      0.000000000000000E+000
>>>>>     Transf. matrix:  0.000000000000000E+000  0.000000000000000E+000
>>>>>       1.00000000000000
>>>>>     operation          16
>>>>>     det:  -1.00000000000000
>>>>> ----------------------------error
>>>>> files---------------------------------------------
>>>>> upoptic.error
>>>>> Error in OPTIC
>>>>> _______________________________________________
>>>>> Wien mailing list
>>>>> Wien at zeus.theochem.tuwien.ac.at
>>>>> http://zeus.theochem.tuwien.ac.at/mailman/listinfo/wien
>>>>> SEARCH the MAILING-LIST at:  http://www.mail-archive.com/wien@zeus.theochem.tuwien.ac.at/index.html
>>>>>
>>>>
>>>> --
>>>> --------------------------------------------------------------------------
>>>> Peter BLAHA, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna
>>>> Phone: +43-1-58801-165300             FAX: +43-1-58801-165982
>>>> Email: blaha at theochem.tuwien.ac.at    WIEN2k: http://www.wien2k.at
>>>> WWW:
>>>> http://www.imc.tuwien.ac.at/tc_blaha-------------------------------------------------------------------------
>>>>
>>>> _______________________________________________
>>>> Wien mailing list
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>>>> http://zeus.theochem.tuwien.ac.at/mailman/listinfo/wien
>>>> SEARCH the MAILING-LIST at:  http://www.mail-archive.com/wien@zeus.theochem.tuwien.ac.at/index.html
>>> _______________________________________________
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>>>
>>
>> --
>>
>>                                         P.Blaha
>> --------------------------------------------------------------------------
>> Peter BLAHA, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna
>> Phone: +43-1-58801-165300             FAX: +43-1-58801-165982
>> Email: blaha at theochem.tuwien.ac.at    WIEN2k: http://www.wien2k.at
>> WWW:   http://www.imc.tuwien.ac.at/TC_Blaha
>> --------------------------------------------------------------------------
>> _______________________________________________
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-- 

                                       P.Blaha
--------------------------------------------------------------------------
Peter BLAHA, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna
Phone: +43-1-58801-165300             FAX: +43-1-58801-165982
Email: blaha at theochem.tuwien.ac.at    WIEN2k: http://www.wien2k.at
WWW:   http://www.imc.tuwien.ac.at/TC_Blaha
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