<div dir="ltr">Dear Prof. Blaha,<br><div><br></div><div>                     Thank you for your advice. However, I have few queryes. For a big cell-like 56 atomic cell semiconductor, can I consider 4 k points during structure optimization while 14 k-points during energy calculation with the optimized structure (<b>the step 4</b>)? If I really need to increase the k-points at the step 4 what should I do?.an initialization with 14 k-points ??</div><div><br></div><div>with regards,</div></div><br><div class="gmail_quote"><div dir="ltr" class="gmail_attr">On Mon, 19 Jul 2021 at 15:30, Peter Blaha <<a href="mailto:pblaha@theochem.tuwien.ac.at">pblaha@theochem.tuwien.ac.at</a>> wrote:<br></div><blockquote class="gmail_quote" style="margin:0px 0px 0px 0.8ex;border-left:1px solid rgb(204,204,204);padding-left:1ex">> (1) runsp_lapw -dm -orb -fc 1.0 -ec 0.0001 -min<br>
> (2) Taking the optimized structure from the previous run, I have started <br>
> force minimization by min-j" runsp_lapw ......<br>
> (3) I have copied the final structure as has been obtained in the force <br>
> minimization & take it to a different directory for simulating the <br>
> energy of the compound.<br>
> (4) By taking the force minimized structure I have run runsp_lapw -dm <br>
> -orb -fc 1.0 -ec 0.0001 -cc 0.0001<br>
> <br>
> Please suggest to me if I am doing something wrong.<br>
<br>
Almost "everything".<br>
<br>
ad 1)  -dm not necessary (-orb will set it automatically); -min DOES <br>
already a force minimization !!!<br>
ad 2) completely unnecessary when you have   -min  in 1)<br>
ad 3) from what you wrote, you only copied case.struct. I'd never do <br>
that, see below.<br>
ad 4)  before you can runsp ..., what have you done ?? You need an <br>
initialization with AFM setup, init_orb<br>
<br>
What you should do (asuming you have a proper initialization):<br>
1)  runsp_lapw -orb -fc 1.0 -ec 0.0001 -min    # check final forces, <br>
otherwise rerun command 1)<br>
2)  save_lapw relaxed<br>
<br>
In case you really want to run another scf in a new directory with the <br>
relaxed structure:<br>
<br>
3) mkdir new; cp relaxed.* new; cd new; restore_lapw relaxed<br>
4) runsp_lapw -orb -fc 1.0 -ec 0.0001<br>
step 4 should stop after 3 cycles.<br>
<br>
> <br>
> warm regards,<br>
> <br>
> <br>
> On Mon, 19 Jul 2021 at 14:47, Peter Blaha <<a href="mailto:pblaha@theochem.tuwien.ac.at" target="_blank">pblaha@theochem.tuwien.ac.at</a> <br>
> <mailto:<a href="mailto:pblaha@theochem.tuwien.ac.at" target="_blank">pblaha@theochem.tuwien.ac.at</a>>> wrote:<br>
> <br>
>      >                    I am working on a frustrated AFM ordering in<br>
>     which<br>
>      > both the atom with spin up & spin down remains at the octahedral<br>
>     site. I<br>
>      > have simulated the same structure with U=4 eV & which works well.<br>
>      > However, when I shifted to U=6 eV the structure showed AFM during<br>
>      > structure optimization while the magnetic moment didn't cancel<br>
>     when I go<br>
>      > for an SCF with the optimized structure.<br>
> <br>
>     When you do "structure optimization  (whatever you actually mean by<br>
>     that<br>
>     ... ?)" you actually do for sure a scf calculation also for the<br>
>     optimized structure. So it seems to work....<br>
> <br>
>     You did not explain what you have done at: "I go for an SCF with the<br>
>     optimized structure".<br>
>     Apparently here you have done something which breaks AFM (it is easy to<br>
>     get some arbitrary magnetic state in DFT+U when one is not careful with<br>
>     dmat* or vorb* files)..<br>
> <br>
> <br>
> <br>
>      ><br>
>      > with regards,<br>
>      ><br>
>      > On Mon, 19 Jul 2021 at 14:32, Laurence Marks<br>
>     <<a href="mailto:laurence.marks@gmail.com" target="_blank">laurence.marks@gmail.com</a> <mailto:<a href="mailto:laurence.marks@gmail.com" target="_blank">laurence.marks@gmail.com</a>><br>
>      > <mailto:<a href="mailto:laurence.marks@gmail.com" target="_blank">laurence.marks@gmail.com</a><br>
>     <mailto:<a href="mailto:laurence.marks@gmail.com" target="_blank">laurence.marks@gmail.com</a>>>> wrote:<br>
>      ><br>
>      >     Without the struct nobody can do more than guess.<br>
>      ><br>
>      >     My guess. In spinel you have any octahedral & tetrahedral<br>
>     sites. You<br>
>      >     put one spin (Up) on octahedral sites, and the other (Dn) on<br>
>      >     tetrahedral. This won't work.<br>
>      ><br>
>      >     _____<br>
>      >     Professor Laurence Marks<br>
>      >     "Research is to see what everybody else has seen, and to<br>
>     think what<br>
>      >     nobody else has thought", Albert Szent-Györgyi<br>
>      > <a href="http://www.numis.northwestern.edu" rel="noreferrer" target="_blank">www.numis.northwestern.edu</a> <<a href="http://www.numis.northwestern.edu" rel="noreferrer" target="_blank">http://www.numis.northwestern.edu</a>><br>
>     <<a href="http://www.numis.northwestern.edu" rel="noreferrer" target="_blank">http://www.numis.northwestern.edu</a> <<a href="http://www.numis.northwestern.edu" rel="noreferrer" target="_blank">http://www.numis.northwestern.edu</a>>><br>
>      ><br>
>      >     On Mon, Jul 19, 2021, 03:23 shamik chakrabarti<br>
>      >     <<a href="mailto:shamik15041981@gmail.com" target="_blank">shamik15041981@gmail.com</a> <mailto:<a href="mailto:shamik15041981@gmail.com" target="_blank">shamik15041981@gmail.com</a>><br>
>     <mailto:<a href="mailto:shamik15041981@gmail.com" target="_blank">shamik15041981@gmail.com</a> <mailto:<a href="mailto:shamik15041981@gmail.com" target="_blank">shamik15041981@gmail.com</a>>>><br>
>     wrote:<br>
>      ><br>
>      >         Dear Wien2k users,<br>
>      ><br>
>      >                              I was running AFM calculation of a<br>
>     spinel<br>
>      >         compound by flipping the spin in case.inst & by running spin<br>
>      >         polarize calculation. During structure optimization, the AFM<br>
>      >         structure appears well with zero moments per unit cell.<br>
>     However,<br>
>      >         when I have started an SCF by taking the<br>
>     optimized structure the<br>
>      >         calculation converges in 50 iterations with a moment ~ 8<br>
>     muB/per<br>
>      >         unit cell. Also, the atoms which are connected with AFM<br>
>     ordering<br>
>      >         do not show equal moments with opposite directions. The<br>
>      >         moment of an atom is 2.7muB while the atom connected with AFM<br>
>      >         ordering showed a moment of -0.77  muB.<br>
>      ><br>
>      >         The convergence criteria was set as: -ec 0.0001, -cc<br>
>     0.0001, fc<br>
>      >         1.0 & the calculation converges in 50 iterations.<br>
>      ><br>
>      >         I have set 14 k-points for 56 atomic cells & also using GGA+U<br>
>      >         with U=6 eV for the TM atom.<br>
>      ><br>
>      >         Any response in this regard will be helpful for us.<br>
>      ><br>
>      >         Thanks in advance,<br>
>      ><br>
>      >         with regards,<br>
>      >         --<br>
>      >         Dr. Shamik Chakrabarti<br>
>      >         Research Fellow<br>
>      >         Department of Physics<br>
>      >         Indian Institute of Technology Patna<br>
>      >         Bihta-801103<br>
>      >         Patna<br>
>      >         Bihar, India<br>
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>      ><br>
>      ><br>
>      ><br>
>      > --<br>
>      > Dr. Shamik Chakrabarti<br>
>      > Research Fellow<br>
>      > Department of Physics<br>
>      > Indian Institute of Technology Patna<br>
>      > Bihta-801103<br>
>      > Patna<br>
>      > Bihar, India<br>
>      ><br>
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>      ><br>
> <br>
>     -- <br>
>     Peter Blaha, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna<br>
>     Phone: +43-1-58801-165300          Email: <a href="mailto:peter.blaha@tuwien.ac.at" target="_blank">peter.blaha@tuwien.ac.at</a><br>
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Peter Blaha, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna<br>
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</blockquote></div><br clear="all"><div><br></div>-- <br><div dir="ltr" class="gmail_signature"><div dir="ltr"><div><div dir="ltr"><div dir="ltr"><div dir="ltr"><div dir="ltr"><div style="font-size:small">Dr. Shamik Chakrabarti</div><div style="font-size:small">Research Fellow </div><div style="font-size:small">Department of Physics</div><div style="font-size:small">Indian Institute of Technology Patna</div><div style="font-size:small">Bihta-801103</div><div style="font-size:small">Patna</div><div style="font-size:small">Bihar, India</div></div></div></div></div></div></div></div>