[Wien] runafm

Peter Blaha pblaha at theochem.tuwien.ac.at
Mon Oct 15 09:55:13 CEST 2007


With the "diamond" example I could verify your problem.

It seems to be connected with the fourier-coefficients, where one should
take the complex conjugate in the transformation.

Please change one line in SRC_clmcopy/clmcopy.f :

              TKK= - TKK*TPI

With this modification it seems to work.

The fix should concern ONLY cases without inversion symmetry and a non-symmorphic
symmetry operation (one with a translation) .


Pablo de la Mora schrieb:
> Dear Peter Blaha,
>    I am surprised, I found that this operation is the one that relates 
> the spins, I ran 'init' and at the end I put this operation, here is the 
> <case>.inclmcopy:
> -----------------------------------
> more init.inclmcopy
>   1                                              NUMBER of ATOMS to CHANGE
>   1   2                                          INTERCHANGE these ATOMS
> -1.00000000000  0.00000000000  0.00000000000    1    0    0 
> 0.00000000     SYMMETRY OPERATION  0.00000000000 -1.00000000000  
> 0.00000000000    0    1    0 0.00000000
>  0.00000000000  0.00000000000 -1.00000000000    0    0    1 0.00000000
>  12                                              NUMBER of LM to CHANGE 
> SIGN
>  1 1    1 1 -1.00
> -1 1   -1 1 -1.00
>  3 1    3 1 -1.00
> -3 1   -3 1 -1.00
>  3 3    3 3 -1.00
> -3 3   -3 3 -1.00
>  5 1    5 1 -1.00
> -5 1   -5 1 -1.00
>  5 3    5 3 -1.00
> -5 3   -5 3 -1.00
>  5 5    5 5 -1.00
> -5 5   -5 5 -1.00
>  -1   0   0   0.50000
>   0  -1   0   0.50000
>   0   0  -1   0.16560
> The symmetry operation above is one of the operations of the NM-supergroup
> missing in the AFM-subgroup (transfers spin-up into spin-dn atom)
> ------------------------------------------------------
> The ferromagnetic case is:
> a=6.845A, b=4.206A, c=7.222A
> SG: 62_Pnma
> U: 0.0101, 0.25, 0.2925
> 
> and the antiferromagneti case is:
> a=4.206A, b=6.845A, c=7.222A
> SG: 31_Pmn21
> U up: 0, 0.2399, 0.2903
> U dn: 0, 0.7399, 0.3753
> as I wrote down.
> 
> I tried with U=>Fe, and the same happens
> I tried Fe in Zincblenda structure
> a=b=c=5.733A
> Fe up: 1/8, 1/8, 1/8
> Fe dn: -1/8, -1/8, -1/8
> here the symmetry operation is
> -1 0 0  0.0
> 0 -1 0  0.0
> 0 0 -1  0.0
> Here runafm does not put charge into the interstitial, runsp does put 
> very small amount of charge into the intersitital, but at the end both 
> seem to give good results,
> 
> At the end what I find is that SG: 32_Pmn21 seems to give problems with 
> runafm
> 
> Here I am attaching the struct, inst and the inclmcopy files for the 
> runafm run,
> the AFM and SP files are the magnetic moments for the runafm and runsp 
> runs.
> 
>    Yours
> 
>             Pablo de la Mora
> 
> Peter Blaha escribió:
>>  > This structure does not have inversion symmetry, the symmetry 
>> operation
>>  > that relates the up and dn spin atoms is
>>  > -1 0 0  0.5
>>  > 0 -1 0  0.5
>>  > 0 0 -1  0.1656
>>
>> This is certainly NOT a valid symmetry operation!
>>
>> How is the structure of the non-magnetic (or ferromagnetic) case ?
>> Are the 4 U equivalent ?
>>
>> Pablo de la Mora schrieb:
>>  
>>> I found a problem with the 'runafm', this program runs fine with Cr, 
>>> but with U in an ortorhombic symmetry and antiferromangetic 
>>> arrangement it does not; it puts magnetic moment into the 
>>> interstitial region.
>>> Below are the struct and inst files
>>> This structure does not have inversion symmetry, the symmetry 
>>> operation that relates the up and dn spin atoms is
>>> -1 0 0  0.5
>>> 0 -1 0  0.5
>>> 0 0 -1  0.1656
>>> running with runsp it gives no magnetic moment in the interstitial, 
>>> but with runafm the moment increases.
>>> grep :MM *scf
>>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
>>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    3.11726
>>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -3.11726
>>> :MMTOT: TOTAL MAGNETIC MOMENT IN CELL   =    0.00000
>>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
>>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.39863
>>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.39863
>>> :MMTOT: TOTAL MAGNETIC MOMENT IN CELL   =    0.00000
>>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -0.01120
>>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.40694
>>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.40694
>>> :MMTOT: TOTAL MAGNETIC MOMENT IN CELL   =   -0.01120
>>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -1.02171
>>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    3.14755
>>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -3.14755
>>> :MMTOT: TOTAL MAGNETIC MOMENT IN CELL   =   -1.02171
>>>
>>> The first two are with runafm and the next ones are with runafm. A 
>>> similar problem happens starting with runafm.
>>>
>>> struct:
>>> Antiferro U
>>> P   LATTICE,NONEQUIV.ATOMS:  231_Pmn21
>>> MODE OF CALC=RELA unit=ang
>>>   7.948191 12.935180 13.647608 90.000000 90.000000 90.000000
>>> ATOM  -1: X=0.50000000 Y=0.76010000 Z=0.79030000
>>>           MULT= 2          ISPLIT= 8
>>>       -1: X=0.00000000 Y=0.23990000 Z=0.29030000
>>> U 1        NPT=  781  R0=0.00000500 RMT=   2.50000   Z: 92.0
>>> LOCAL ROT MATRIX:    0.0000000 0.0000000 1.0000000
>>>                      1.0000000 0.0000000 0.0000000
>>>                      0.0000000 1.0000000 0.0000000
>>> ATOM  -2: X=0.00000000 Y=0.73990000 Z=0.37530000
>>>           MULT= 2          ISPLIT= 8
>>>       -2: X=0.50000000 Y=0.26010000 Z=0.87530000
>>> U 2        NPT=  781  R0=0.00000500 RMT=   2.50000   Z: 92.0
>>> LOCAL ROT MATRIX:    0.0000000 0.0000000 1.0000000
>>>                      1.0000000 0.0000000 0.0000000
>>>                      0.0000000 1.0000000 0.0000000
>>>    4      NUMBER OF SYMMETRY OPERATIONS
>>> -1 0 0 0.00000000
>>>  0 1 0 0.00000000
>>>  0 0 1 0.00000000
>>>        1
>>>  1 0 0 0.00000000
>>>  0 1 0 0.00000000
>>>  0 0 1 0.00000000
>>>        2
>>> -1 0 0 0.50000000
>>>  0-1 0 0.00000000
>>>  0 0 1 0.50000000
>>>        3
>>>  1 0 0 0.50000000
>>>  0-1 0 0.00000000
>>>  0 0 1 0.50000000
>>>        4
>>>
>>> inst
>>> U 1
>>> Rn 3
>>> 5, 3,3.0  N
>>> 5, 3,0.0  N
>>> 6, 2,1.0  N
>>> 6, 2,0.0  N
>>> 7,-1,1.0  N
>>> 7,-1,1.0  N
>>> U 2
>>> Rn 3
>>> 5, 3,0.0  N
>>> 5, 3,3.0  N
>>> 6, 2,0.0  N
>>> 6, 2,1.0  N
>>> 7,-1,1.0  N
>>> 7,-1,1.0  N
>>> ****     End of Input
>>> ****     End of Input
>>>
>>> _______________________________________________
>>> Wien mailing list
>>> Wien at zeus.theochem.tuwien.ac.at
>>> http://zeus.theochem.tuwien.ac.at/mailman/listinfo/wien
>>>     
>>
>>   
> 
> 
> ------------------------------------------------------------------------
> 
> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -0.06035
> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    3.08708
> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -3.08708
> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -1.50470
> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.15148
> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.15148
> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -0.61138
> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.74360
> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.74360
> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -0.60715
> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.78212
> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.78212
> 
> 
> ------------------------------------------------------------------------
> 
> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    3.08708
> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -3.08708
> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.05272
> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.05272
> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.72067
> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.72067
> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.74278
> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.74279
> 
> 
> ------------------------------------------------------------------------
> 
> Fe 1       
> Ar 3  
> 3, 2,2.0  N
> 3, 2,2.0  N
> 3,-3,2.5  N
> 3,-3,0.0  N
> 4,-1,1.0  N
> 4,-1,0.5  N
> Fe 2       
> Ar 3  
> 3, 2,2.0  N
> 3, 2,2.0  N
> 3,-3,0.0  N
> 3,-3,2.5  N
> 4,-1,0.5  N
> 4,-1,1.0  N
> ****     End of Input
> ****     End of Input
> 
> 
> ------------------------------------------------------------------------
> 
> Superconductor magnético UCoGe                                                 
> P   LATTICE,NONEQUIV.ATOMS:  231_Pmn21                                         
> MODE OF CALC=RELA unit=ang                                                     
>   7.948191 12.935180 13.647608 90.000000 90.000000 90.000000                   
> ATOM  -1: X=0.50000000 Y=0.76010000 Z=0.79030000
>           MULT= 2          ISPLIT= 8
>       -1: X=0.00000000 Y=0.23990000 Z=0.29030000
> Fe1        NPT=  781  R0=0.00005000 RMT=   2.50000   Z: 26.0                   
> LOCAL ROT MATRIX:    0.0000000 0.0000000 1.0000000
>                      1.0000000 0.0000000 0.0000000
>                      0.0000000 1.0000000 0.0000000
> ATOM  -2: X=0.00000000 Y=0.73990000 Z=0.37530000
>           MULT= 2          ISPLIT= 8
>       -2: X=0.50000000 Y=0.26010000 Z=0.87530000
> Fe2        NPT=  781  R0=0.00005000 RMT=   2.50000   Z: 26.0                   
> LOCAL ROT MATRIX:    0.0000000 0.0000000 1.0000000
>                      1.0000000 0.0000000 0.0000000
>                      0.0000000 1.0000000 0.0000000
>    4      NUMBER OF SYMMETRY OPERATIONS
> -1 0 0 0.00000000
>  0 1 0 0.00000000
>  0 0 1 0.00000000
>        1
>  1 0 0 0.00000000
>  0 1 0 0.00000000
>  0 0 1 0.00000000
>        2
> -1 0 0 0.50000000
>  0-1 0 0.00000000
>  0 0 1 0.50000000
>        3
>  1 0 0 0.50000000
>  0-1 0 0.00000000
>  0 0 1 0.50000000
>        4
> 
> 
> ------------------------------------------------------------------------
> 
>    1                                              NUMBER of ATOMS to CHANGE
>    1   2                                          INTERCHANGE these ATOMS
>  -1.00000000000  0.00000000000  0.00000000000    1    0    0 0.00000000     SYMMETRY OPERATION
>   0.00000000000 -1.00000000000  0.00000000000    0    1    0 0.00000000
>   0.00000000000  0.00000000000 -1.00000000000    0    0    1 0.00000000
>   12                                              NUMBER of LM to CHANGE SIGN
>   1 1    1 1 -1.00
>  -1 1   -1 1 -1.00
>   3 1    3 1 -1.00
>  -3 1   -3 1 -1.00
>   3 3    3 3 -1.00
>  -3 3   -3 3 -1.00
>   5 1    5 1 -1.00
>  -5 1   -5 1 -1.00
>   5 3    5 3 -1.00
>  -5 3   -5 3 -1.00
>   5 5    5 5 -1.00
>  -5 5   -5 5 -1.00
>   -1   0   0   0.50000
>    0  -1   0   0.50000
>    0   0  -1   0.16560
>  The symmetry operation above is one of the operations of the NM-supergroup
>  missing in the AFM-subgroup (transfers spin-up into spin-dn atom)
> 
> 
> ------------------------------------------------------------------------
> 
> _______________________________________________
> Wien mailing list
> Wien at zeus.theochem.tuwien.ac.at
> http://zeus.theochem.tuwien.ac.at/mailman/listinfo/wien

-- 

                                       P.Blaha
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Peter BLAHA, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna
Phone: +43-1-58801-15671             FAX: +43-1-58801-15698
Email: blaha at theochem.tuwien.ac.at    WWW: http://info.tuwien.ac.at/theochem/
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