[Wien] runafm

Pablo de la Mora delamora at servidor.unam.mx
Thu Oct 25 16:20:37 CEST 2007


Dr. Blaha,
    Thank you for this correction, now I can run 'runafm' in systems 
without inversion symmetry. After convergency I checked with 'runsp' and 
it was OK.
    I would like to comment that I am glad that the latest version 7.3 
now accepts 'runafm -orb' which I think was not implemented earlier.
    Also this version seems more friendly; it gives more information of 
what is going wrong;
I had the files
    <case>.indm
    <case>.inorb
but since the system didn't have inversion symmetry, it needed complex 
algebra and the file
   <case>.indm
needed to be changed to
   <case>.indmc
with this the runafm -orb ran without problems.

          Pablo de la Mora

Peter Blaha escribió:
> With the "diamond" example I could verify your problem.
>
> It seems to be connected with the fourier-coefficients, where one should
> take the complex conjugate in the transformation.
>
> Please change one line in SRC_clmcopy/clmcopy.f :
>
>               TKK= - TKK*TPI
>
> With this modification it seems to work.
>
> The fix should concern ONLY cases without inversion symmetry and a non-symmorphic
> symmetry operation (one with a translation) .
>
>
> Pablo de la Mora schrieb:
>   
>> Dear Peter Blaha,
>>    I am surprised, I found that this operation is the one that relates 
>> the spins, I ran 'init' and at the end I put this operation, here is the 
>> <case>.inclmcopy:
>> -----------------------------------
>> more init.inclmcopy
>>   1                                              NUMBER of ATOMS to CHANGE
>>   1   2                                          INTERCHANGE these ATOMS
>> -1.00000000000  0.00000000000  0.00000000000    1    0    0 
>> 0.00000000     SYMMETRY OPERATION  0.00000000000 -1.00000000000  
>> 0.00000000000    0    1    0 0.00000000
>>  0.00000000000  0.00000000000 -1.00000000000    0    0    1 0.00000000
>>  12                                              NUMBER of LM to CHANGE 
>> SIGN
>>  1 1    1 1 -1.00
>> -1 1   -1 1 -1.00
>>  3 1    3 1 -1.00
>> -3 1   -3 1 -1.00
>>  3 3    3 3 -1.00
>> -3 3   -3 3 -1.00
>>  5 1    5 1 -1.00
>> -5 1   -5 1 -1.00
>>  5 3    5 3 -1.00
>> -5 3   -5 3 -1.00
>>  5 5    5 5 -1.00
>> -5 5   -5 5 -1.00
>>  -1   0   0   0.50000
>>   0  -1   0   0.50000
>>   0   0  -1   0.16560
>> The symmetry operation above is one of the operations of the NM-supergroup
>> missing in the AFM-subgroup (transfers spin-up into spin-dn atom)
>> ------------------------------------------------------
>> The ferromagnetic case is:
>> a=6.845A, b=4.206A, c=7.222A
>> SG: 62_Pnma
>> U: 0.0101, 0.25, 0.2925
>>
>> and the antiferromagneti case is:
>> a=4.206A, b=6.845A, c=7.222A
>> SG: 31_Pmn21
>> U up: 0, 0.2399, 0.2903
>> U dn: 0, 0.7399, 0.3753
>> as I wrote down.
>>
>> I tried with U=>Fe, and the same happens
>> I tried Fe in Zincblenda structure
>> a=b=c=5.733A
>> Fe up: 1/8, 1/8, 1/8
>> Fe dn: -1/8, -1/8, -1/8
>> here the symmetry operation is
>> -1 0 0  0.0
>> 0 -1 0  0.0
>> 0 0 -1  0.0
>> Here runafm does not put charge into the interstitial, runsp does put 
>> very small amount of charge into the intersitital, but at the end both 
>> seem to give good results,
>>
>> At the end what I find is that SG: 32_Pmn21 seems to give problems with 
>> runafm
>>
>> Here I am attaching the struct, inst and the inclmcopy files for the 
>> runafm run,
>> the AFM and SP files are the magnetic moments for the runafm and runsp 
>> runs.
>>
>>    Yours
>>
>>             Pablo de la Mora
>>
>> Peter Blaha escribió:
>>     
>>>  > This structure does not have inversion symmetry, the symmetry 
>>> operation
>>>  > that relates the up and dn spin atoms is
>>>  > -1 0 0  0.5
>>>  > 0 -1 0  0.5
>>>  > 0 0 -1  0.1656
>>>
>>> This is certainly NOT a valid symmetry operation!
>>>
>>> How is the structure of the non-magnetic (or ferromagnetic) case ?
>>> Are the 4 U equivalent ?
>>>
>>> Pablo de la Mora schrieb:
>>>  
>>>       
>>>> I found a problem with the 'runafm', this program runs fine with Cr, 
>>>> but with U in an ortorhombic symmetry and antiferromangetic 
>>>> arrangement it does not; it puts magnetic moment into the 
>>>> interstitial region.
>>>> Below are the struct and inst files
>>>> This structure does not have inversion symmetry, the symmetry 
>>>> operation that relates the up and dn spin atoms is
>>>> -1 0 0  0.5
>>>> 0 -1 0  0.5
>>>> 0 0 -1  0.1656
>>>> running with runsp it gives no magnetic moment in the interstitial, 
>>>> but with runafm the moment increases.
>>>> grep :MM *scf
>>>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
>>>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    3.11726
>>>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -3.11726
>>>> :MMTOT: TOTAL MAGNETIC MOMENT IN CELL   =    0.00000
>>>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
>>>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.39863
>>>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.39863
>>>> :MMTOT: TOTAL MAGNETIC MOMENT IN CELL   =    0.00000
>>>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -0.01120
>>>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.40694
>>>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.40694
>>>> :MMTOT: TOTAL MAGNETIC MOMENT IN CELL   =   -0.01120
>>>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -1.02171
>>>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    3.14755
>>>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -3.14755
>>>> :MMTOT: TOTAL MAGNETIC MOMENT IN CELL   =   -1.02171
>>>>
>>>> The first two are with runafm and the next ones are with runafm. A 
>>>> similar problem happens starting with runafm.
>>>>
>>>> struct:
>>>> Antiferro U
>>>> P   LATTICE,NONEQUIV.ATOMS:  231_Pmn21
>>>> MODE OF CALC=RELA unit=ang
>>>>   7.948191 12.935180 13.647608 90.000000 90.000000 90.000000
>>>> ATOM  -1: X=0.50000000 Y=0.76010000 Z=0.79030000
>>>>           MULT= 2          ISPLIT= 8
>>>>       -1: X=0.00000000 Y=0.23990000 Z=0.29030000
>>>> U 1        NPT=  781  R0=0.00000500 RMT=   2.50000   Z: 92.0
>>>> LOCAL ROT MATRIX:    0.0000000 0.0000000 1.0000000
>>>>                      1.0000000 0.0000000 0.0000000
>>>>                      0.0000000 1.0000000 0.0000000
>>>> ATOM  -2: X=0.00000000 Y=0.73990000 Z=0.37530000
>>>>           MULT= 2          ISPLIT= 8
>>>>       -2: X=0.50000000 Y=0.26010000 Z=0.87530000
>>>> U 2        NPT=  781  R0=0.00000500 RMT=   2.50000   Z: 92.0
>>>> LOCAL ROT MATRIX:    0.0000000 0.0000000 1.0000000
>>>>                      1.0000000 0.0000000 0.0000000
>>>>                      0.0000000 1.0000000 0.0000000
>>>>    4      NUMBER OF SYMMETRY OPERATIONS
>>>> -1 0 0 0.00000000
>>>>  0 1 0 0.00000000
>>>>  0 0 1 0.00000000
>>>>        1
>>>>  1 0 0 0.00000000
>>>>  0 1 0 0.00000000
>>>>  0 0 1 0.00000000
>>>>        2
>>>> -1 0 0 0.50000000
>>>>  0-1 0 0.00000000
>>>>  0 0 1 0.50000000
>>>>        3
>>>>  1 0 0 0.50000000
>>>>  0-1 0 0.00000000
>>>>  0 0 1 0.50000000
>>>>        4
>>>>
>>>> inst
>>>> U 1
>>>> Rn 3
>>>> 5, 3,3.0  N
>>>> 5, 3,0.0  N
>>>> 6, 2,1.0  N
>>>> 6, 2,0.0  N
>>>> 7,-1,1.0  N
>>>> 7,-1,1.0  N
>>>> U 2
>>>> Rn 3
>>>> 5, 3,0.0  N
>>>> 5, 3,3.0  N
>>>> 6, 2,0.0  N
>>>> 6, 2,1.0  N
>>>> 7,-1,1.0  N
>>>> 7,-1,1.0  N
>>>> ****     End of Input
>>>> ****     End of Input
>>>>
>>>> _______________________________________________
>>>> Wien mailing list
>>>> Wien at zeus.theochem.tuwien.ac.at
>>>> http://zeus.theochem.tuwien.ac.at/mailman/listinfo/wien
>>>>     
>>>>         
>>>   
>>>       
>> ------------------------------------------------------------------------
>>
>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -0.06035
>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    3.08708
>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -3.08708
>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -1.50470
>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.15148
>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.15148
>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -0.61138
>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.74360
>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.74360
>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =   -0.60715
>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.78212
>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.78212
>>
>>
>> ------------------------------------------------------------------------
>>
>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    3.08708
>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -3.08708
>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.05272
>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.05272
>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.72067
>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.72067
>> :MMINT: MAGNETIC MOMENT IN INTERSTITIAL =    0.00000
>> :MMI001: MAGNETIC MOMENT IN SPHERE   1    =    2.74278
>> :MMI002: MAGNETIC MOMENT IN SPHERE   2    =   -2.74279
>>
>>
>> ------------------------------------------------------------------------
>>
>> Fe 1       
>> Ar 3  
>> 3, 2,2.0  N
>> 3, 2,2.0  N
>> 3,-3,2.5  N
>> 3,-3,0.0  N
>> 4,-1,1.0  N
>> 4,-1,0.5  N
>> Fe 2       
>> Ar 3  
>> 3, 2,2.0  N
>> 3, 2,2.0  N
>> 3,-3,0.0  N
>> 3,-3,2.5  N
>> 4,-1,0.5  N
>> 4,-1,1.0  N
>> ****     End of Input
>> ****     End of Input
>>
>>
>> ------------------------------------------------------------------------
>>
>> Superconductor magnético UCoGe                                                 
>> P   LATTICE,NONEQUIV.ATOMS:  231_Pmn21                                         
>> MODE OF CALC=RELA unit=ang                                                     
>>   7.948191 12.935180 13.647608 90.000000 90.000000 90.000000                   
>> ATOM  -1: X=0.50000000 Y=0.76010000 Z=0.79030000
>>           MULT= 2          ISPLIT= 8
>>       -1: X=0.00000000 Y=0.23990000 Z=0.29030000
>> Fe1        NPT=  781  R0=0.00005000 RMT=   2.50000   Z: 26.0                   
>> LOCAL ROT MATRIX:    0.0000000 0.0000000 1.0000000
>>                      1.0000000 0.0000000 0.0000000
>>                      0.0000000 1.0000000 0.0000000
>> ATOM  -2: X=0.00000000 Y=0.73990000 Z=0.37530000
>>           MULT= 2          ISPLIT= 8
>>       -2: X=0.50000000 Y=0.26010000 Z=0.87530000
>> Fe2        NPT=  781  R0=0.00005000 RMT=   2.50000   Z: 26.0                   
>> LOCAL ROT MATRIX:    0.0000000 0.0000000 1.0000000
>>                      1.0000000 0.0000000 0.0000000
>>                      0.0000000 1.0000000 0.0000000
>>    4      NUMBER OF SYMMETRY OPERATIONS
>> -1 0 0 0.00000000
>>  0 1 0 0.00000000
>>  0 0 1 0.00000000
>>        1
>>  1 0 0 0.00000000
>>  0 1 0 0.00000000
>>  0 0 1 0.00000000
>>        2
>> -1 0 0 0.50000000
>>  0-1 0 0.00000000
>>  0 0 1 0.50000000
>>        3
>>  1 0 0 0.50000000
>>  0-1 0 0.00000000
>>  0 0 1 0.50000000
>>        4
>>
>>
>> ------------------------------------------------------------------------
>>
>>    1                                              NUMBER of ATOMS to CHANGE
>>    1   2                                          INTERCHANGE these ATOMS
>>  -1.00000000000  0.00000000000  0.00000000000    1    0    0 0.00000000     SYMMETRY OPERATION
>>   0.00000000000 -1.00000000000  0.00000000000    0    1    0 0.00000000
>>   0.00000000000  0.00000000000 -1.00000000000    0    0    1 0.00000000
>>   12                                              NUMBER of LM to CHANGE SIGN
>>   1 1    1 1 -1.00
>>  -1 1   -1 1 -1.00
>>   3 1    3 1 -1.00
>>  -3 1   -3 1 -1.00
>>   3 3    3 3 -1.00
>>  -3 3   -3 3 -1.00
>>   5 1    5 1 -1.00
>>  -5 1   -5 1 -1.00
>>   5 3    5 3 -1.00
>>  -5 3   -5 3 -1.00
>>   5 5    5 5 -1.00
>>  -5 5   -5 5 -1.00
>>   -1   0   0   0.50000
>>    0  -1   0   0.50000
>>    0   0  -1   0.16560
>>  The symmetry operation above is one of the operations of the NM-supergroup
>>  missing in the AFM-subgroup (transfers spin-up into spin-dn atom)
>>
>>
>> ------------------------------------------------------------------------
>>
>> _______________________________________________
>> Wien mailing list
>> Wien at zeus.theochem.tuwien.ac.at
>> http://zeus.theochem.tuwien.ac.at/mailman/listinfo/wien
>>     
>
>   



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