[Wien] MBJ, case.in0_grr

shima pourrad shima.pourrad at gmail.com
Mon Dec 21 08:13:48 CET 2015


Dear Tran

Yes . I ran it again and achieved the same results with the two different
case.in0_grr .

(sorry for my delay )
Thanks a lot.
Shima M.Pourrad

On Sat, Dec 19, 2015 at 11:28 AM, <tran at theochem.tuwien.ac.at> wrote:

> I don' fully understand you explanantions. Finally, are the results
> with the two different case.in0_grr the same?
>
>
> On Sat, 19 Dec 2015, shima pourrad wrote:
>
>
>> Dear Tran
>>
>> I ran the calculations with “i 200” to increase the default iterations,
>> but I don’t know why my second calculation leads to different results! I
>> ran it again (with MSR1) and it gave me
>> the same results of the first calculation (with PRATT). Now, there are
>> not any ambiguities for me. I appreciate a lot because of your explanation
>> again.
>>
>> Sincerely yours.
>>
>> Shima M.Pourrad
>>
>> On Wed, Dec 16, 2015 at 12:26 PM, <tran at theochem.tuwien.ac.at> wrote:
>>       Hi,
>>
>>       MSR1 and PRATT (not PRRAT) should obviously lead to the same results
>>       as long as you let the calculations run until they are sufficiently
>>       well converged. By default a calculation stops after 40 iterations
>>       even if the convergence criteria are not reached. Execute run_lapw
>> with
>>       option "-i 100" to increase to 100 for instance.
>>
>>       Usually, I start with MSR1. If the calculation
>>       does not seem to converge with MSR1 (infinite oscillations or
>> diverge),
>>       I stop the calculation. Then, I restart the calculation with
>>       PRATT with a very small mixing factor like 0.05 and regenerate
>>       case.clmsum with dstart or from previous PBE calculation.
>>       Then, if the calculation seems to converge, I switch back to default
>>       parameters in case.inm to reach convergence a little bit faster.
>>
>>       F. Tran
>>
>>       On Wed, 16 Dec 2015, shima pourrad wrote:
>>
>>
>>             Dear F.Tran
>>
>>             I appreciate a lot because of your explanation. I ran the
>> calculations with  -ec 0.00001 convergence criteria. But unfortunately I
>>             found that I made a bad mistake : for the second calculation
>> I forgot to change the mixing scheme to PRRAT , and it ran with the
>>             default mixing scheme which is MSR1. And this mistake causes
>> two different results.(When I corrected mixing scheme , both
>>             calculations gave me the same results ). I apologize because
>> of this carelessness.
>>
>>             So I have another question, which of the two mixing schemes
>> gives me reliable results? I mean, is it possible my first calculation
>>             (with PRRAT and mixing factor=0.2) converged to the ghost
>> band??  In user guide it was written that: in most cases it is possible
>>             to switch back to MSR1 after some initial scf-cycles. Can we
>> use MSR1 from the first of the calculation? What kind of mixing scheme
>>             we can use for the mbj calculations?
>>
>>             Thanks a lot.
>>
>>             Shima M.pourrad
>>
>>
>>             On Mon, Dec 14, 2015 at 7:39 PM, <tran at theochem.tuwien.ac.at>
>> wrote:
>>                   For the moment, I suspect that your calculations are
>> not very well
>>                   converged. Did you run the calculations with good
>> energy and charge
>>                   convergence criteria? If not, run the two calculations
>> with
>>                   -ec 0.0001 -cc 0.0001
>>                   which is fairly good criteria. Then, maybe the two
>> calculations
>>                   give same results.
>>
>>
>>                   On Mon, 14 Dec 2015, shima pourrad wrote:
>>
>>
>>                         Hi
>>
>>                         Thanks for your prompt answer.
>>
>>                         Yes, for the first calculation with “ EX_GRR
>> VX_GRR” I have :
>>
>>                         Case.in0 :
>>
>>                         TOT  XC_MBJ
>> (XC_LDA,XC_PBESOL,XC_WC,XC_MBJ,XC_REVTPSS)
>>
>>                         R2V      IFFT      (R2V)
>>
>>                          120 120 120    1.00  1    min IFFT-parameters,
>> enhancement factor, iprint
>>
>>
>>
>>                         And case.in0_grr :
>>
>>                         TOT  EX_GRR VX_GRR
>> (XC_LDA,XC_PBESOL,XC_WC,XC_MBJ,XC_REVTPSS)
>>
>>                         R2V      IFFT      (R2V)
>>
>>                          120 120 120    1.00  1    min IFFT-parameters,
>> enhancement factor, iprint
>>
>>
>>
>>                          This calculation give me these results by
>> Analysis :
>>
>>                         --- ENE -----------
>>
>>                         in  1 files:
>>
>>                         case.scf::ENE  : *WARNING** TOTAL ENERGY IN Ry
>> =       -79386.93188247
>>
>>                         --- FER -----------
>>
>>                         in  1 files:
>>
>>                         case.scf::FER  : F E R M I - ENERGY(TETRAH.M.)=
>> 0.4117108915
>>
>>                         --- GAP -----------
>>
>>                         in  1 files:
>>
>>                         case.scf::GAP  :    0.0564 Ry =     0.767 eV
>> (provided you have a proper k-mesh)
>>
>>
>>
>>                         For the second calculation with “ EX_GRR EC_NONE
>> VX_GRR VC_NONE” I have:
>>
>>                         Case.in0 :
>>
>>                         TOT   XC_MBJ (
>> (XC_LDA,XC_PBESOL,XC_WC,XC_MBJ,XC_REVTPSS)
>>
>>                         R2V      IFFT      (R2V)
>>
>>                          120 120 120    1.00  1    min IFFT-parameters,
>> enhancement factor, iprint
>>
>>
>>
>>                         And case.in0_grr :
>>
>>                         TOT   EX_GRR EC_NONE VX_GRR VC_NONE (
>> (XC_LDA,XC_PBESOL,XC_WC,XC_MBJ,XC_REVTPSS)
>>
>>                         R2V      IFFT      (R2V)
>>
>>                          120 120 120    1.00  1    min IFFT-parameters,
>> enhancement factor, iprint
>>
>>
>>
>>
>>
>>                         And its results :
>>
>>                         --- ENE -----------
>>
>>                         in  1 files:
>>
>>                         case.scf::ENE  : *WARNING** TOTAL ENERGY IN Ry
>> =       -79386.93585459
>>
>>                         --- FER -----------
>>
>>                         in  1 files:
>>
>>                         case.scf::FER  : F E R M I - ENERGY(TETRAH.M.)=
>>  0.4269866858
>>
>>                         --- GAP -----------
>>
>>                         in  1 files:
>>
>>                         case.scf::GAP  :    0.0423 Ry =     0.575 eV
>> (provided you have a proper k-mesh)
>>
>>
>>
>>                         what is your opinion?
>>
>>                         Sincerely
>>
>>                         Shima M.Pourrad
>>
>>
>>                         On Mon, Dec 14, 2015 at 6:11 PM, <
>> tran at theochem.tuwien.ac.at> wrote:
>>                               Hi,
>>
>>                               "XC_MBJ" in the 1st line of case.in0
>> indicates that the mBJ method
>>                               will be used. For mBJ, it is necessary to
>> have also the file case.in0_grr
>>                               such that the average of grad(rho)/rho in
>> the unit cell
>>                               [used for Eq. (3) in PRL 102, 226401
>> (2009)] is calculated.
>>
>>                               According to a test that I've just made it
>> does not matter which one
>>                               of these two is specified in case.in0_grr:
>>                               "EX_GRR EC_NONE VX_GRR VC_NONE"
>>                               "EX_GRR VX_GRR"
>>
>>                               So, I don't understand why you got two
>> different results.
>>                               Can you show us the input files case.in0
>> and case.in0_grr
>>                               that you used for the two calculations?
>>
>>                               F. Tran
>>
>>                               On Mon, 14 Dec 2015, shima pourrad wrote:
>>
>>
>>                                     Dear P.Blaha and F.Tran and Wien2k
>> Users
>>
>>                                     I am running wien version14.2 .The
>> purpose of my calculations is to get accurate gap and band
>>                         structure. Hence I am performing MBJ calculations
>> with the parameters special to semiconductors.
>>
>>                                     I would like to ask how we should
>> edit case.in0_grr for a mbj calculation in wien2k14.2 ?
>>
>>                                     I read the user guide and checked the
>> mailing list before, I didn’t find any obvious
>>                         instruction.
>>
>>                                     In user guide, it was written that:
>> when you perform init_mbj_lapw for the second time, some
>>                         steps must do automatically:
>>
>>                                      *
>>                                         edit case.in0 and change the
>> functional to option XC_MBJ. (ok this step is done).
>>
>>                                      *
>>                                          cp case.in0 case.in0_grr and
>> choose EX_GRR VX_GRR in case.in0_grr.
>>
>>                                     But this step, when I open the
>> case.in0_grr to check that, at first line, it was written that:
>>                         EX_GRR EC_NONE VX_GRR VC_NONE. Is it a correct
>> edition? Should I remove “EC_NONE VC_NONE” from the first
>>                         line?
>>
>>                                     I think “EX_GRR EC_NONE VX_GRR
>> VC_NONE” means that correlation energy and potential are
>>                         ignored! But “EX_GRR VX_GRR” alone, means there
>> is a kind of correlation energy and potential as a default
>>                         for usual mbj calculation. Did I realize
>>                                     correctly??
>>
>>                                     You answered the question about the
>> use of the PBE instead of LDA for the energy before:
>>
>> http://www.mail-archive.com/wien%40zeus.theochem.tuwien.ac.at/msg13395.html
>>
>>                                     And it is stated that how we must
>> change case.in0 .
>>
>>                                     But there is no instruction for
>> case.in0_grr. What should be done for this issue?
>>
>>                                     (What kind of edition is correct for
>> case.in0_grr? “EX_GRR VX_GRR”? Or “ EX_GRR EC_NONE VX_GRR
>>                         VC_NONE”?? I performed both of them for one
>> structure, and got very different result: different Gaps,
>>                         different total energies and different
>>                                     Fermi-energies!!! )
>>
>>                                     Please help me.
>>
>>                                     Sincerely
>>
>>                                     Shima M.Pourrad
>>
>>                                     PhD student of physics in condensed
>> matter
>>
>>                                     Science and Research Branch
>>                                     Islamic Azad University
>>
>>
>>
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