[Wien] MBJ, case.in0_grr

tran at theochem.tuwien.ac.at tran at theochem.tuwien.ac.at
Sat Dec 19 08:58:09 CET 2015


I don' fully understand you explanantions. Finally, are the results
with the two different case.in0_grr the same?

On Sat, 19 Dec 2015, shima pourrad wrote:

> 
> Dear Tran
> 
> I ran the calculations with “i 200” to increase the default iterations, but I don’t know why my second calculation leads to different results! I ran it again (with MSR1) and it gave me
> the same results of the first calculation (with PRATT). Now, there are not any ambiguities for me. I appreciate a lot because of your explanation again.
> 
> Sincerely yours.
> 
> Shima M.Pourrad
> 
> On Wed, Dec 16, 2015 at 12:26 PM, <tran at theochem.tuwien.ac.at> wrote:
>       Hi,
>
>       MSR1 and PRATT (not PRRAT) should obviously lead to the same results
>       as long as you let the calculations run until they are sufficiently
>       well converged. By default a calculation stops after 40 iterations
>       even if the convergence criteria are not reached. Execute run_lapw with
>       option "-i 100" to increase to 100 for instance.
>
>       Usually, I start with MSR1. If the calculation
>       does not seem to converge with MSR1 (infinite oscillations or diverge),
>       I stop the calculation. Then, I restart the calculation with
>       PRATT with a very small mixing factor like 0.05 and regenerate
>       case.clmsum with dstart or from previous PBE calculation.
>       Then, if the calculation seems to converge, I switch back to default
>       parameters in case.inm to reach convergence a little bit faster.
>
>       F. Tran
>
>       On Wed, 16 Dec 2015, shima pourrad wrote:
> 
>
>             Dear F.Tran
>
>             I appreciate a lot because of your explanation. I ran the calculations with  -ec 0.00001 convergence criteria. But unfortunately I
>             found that I made a bad mistake : for the second calculation I forgot to change the mixing scheme to PRRAT , and it ran with the
>             default mixing scheme which is MSR1. And this mistake causes two different results.(When I corrected mixing scheme , both
>             calculations gave me the same results ). I apologize because of this carelessness.
>
>             So I have another question, which of the two mixing schemes gives me reliable results? I mean, is it possible my first calculation
>             (with PRRAT and mixing factor=0.2) converged to the ghost band??  In user guide it was written that: in most cases it is possible
>             to switch back to MSR1 after some initial scf-cycles. Can we use MSR1 from the first of the calculation? What kind of mixing scheme
>             we can use for the mbj calculations?  
>
>             Thanks a lot.
>
>             Shima M.pourrad
> 
>
>             On Mon, Dec 14, 2015 at 7:39 PM, <tran at theochem.tuwien.ac.at> wrote:
>                   For the moment, I suspect that your calculations are not very well
>                   converged. Did you run the calculations with good energy and charge
>                   convergence criteria? If not, run the two calculations with
>                   -ec 0.0001 -cc 0.0001
>                   which is fairly good criteria. Then, maybe the two calculations
>                   give same results.
> 
>
>                   On Mon, 14 Dec 2015, shima pourrad wrote:
> 
>
>                         Hi
>
>                         Thanks for your prompt answer.
>
>                         Yes, for the first calculation with “ EX_GRR VX_GRR” I have :
>
>                         Case.in0 :
>
>                         TOT  XC_MBJ     (XC_LDA,XC_PBESOL,XC_WC,XC_MBJ,XC_REVTPSS)                     
>
>                         R2V      IFFT      (R2V)
>
>                          120 120 120    1.00  1    min IFFT-parameters, enhancement factor, iprint
>
>                          
>
>                         And case.in0_grr :
>
>                         TOT  EX_GRR VX_GRR     (XC_LDA,XC_PBESOL,XC_WC,XC_MBJ,XC_REVTPSS)                     
>
>                         R2V      IFFT      (R2V)
>
>                          120 120 120    1.00  1    min IFFT-parameters, enhancement factor, iprint
>
>                          
>
>                          This calculation give me these results by Analysis :
>
>                         --- ENE -----------
>
>                         in  1 files:
>
>                         case.scf::ENE  : *WARNING** TOTAL ENERGY IN Ry =       -79386.93188247
>
>                         --- FER -----------
>
>                         in  1 files:
>
>                         case.scf::FER  : F E R M I - ENERGY(TETRAH.M.)=   0.4117108915
>
>                         --- GAP -----------
>
>                         in  1 files:
>
>                         case.scf::GAP  :    0.0564 Ry =     0.767 eV   (provided you have a proper k-mesh)
>
>                          
>
>                         For the second calculation with “ EX_GRR EC_NONE VX_GRR VC_NONE” I have:
>
>                         Case.in0 :
>
>                         TOT   XC_MBJ (  (XC_LDA,XC_PBESOL,XC_WC,XC_MBJ,XC_REVTPSS)                     
>
>                         R2V      IFFT      (R2V)
>
>                          120 120 120    1.00  1    min IFFT-parameters, enhancement factor, iprint
>
>                          
>
>                         And case.in0_grr :
>
>                         TOT   EX_GRR EC_NONE VX_GRR VC_NONE (  (XC_LDA,XC_PBESOL,XC_WC,XC_MBJ,XC_REVTPSS)                     
>
>                         R2V      IFFT      (R2V)
>
>                          120 120 120    1.00  1    min IFFT-parameters, enhancement factor, iprint
>
>                          
>
>                          
>
>                         And its results :
>
>                         --- ENE -----------
>
>                         in  1 files:
>
>                         case.scf::ENE  : *WARNING** TOTAL ENERGY IN Ry =       -79386.93585459
>
>                         --- FER -----------
>
>                         in  1 files:
>
>                         case.scf::FER  : F E R M I - ENERGY(TETRAH.M.)=   0.4269866858
>
>                         --- GAP -----------
>
>                         in  1 files:
>
>                         case.scf::GAP  :    0.0423 Ry =     0.575 eV   (provided you have a proper k-mesh)
>
>                          
>
>                         what is your opinion?
>
>                         Sincerely
>
>                         Shima M.Pourrad
> 
>
>                         On Mon, Dec 14, 2015 at 6:11 PM, <tran at theochem.tuwien.ac.at> wrote:
>                               Hi,
>
>                               "XC_MBJ" in the 1st line of case.in0 indicates that the mBJ method
>                               will be used. For mBJ, it is necessary to have also the file case.in0_grr
>                               such that the average of grad(rho)/rho in the unit cell
>                               [used for Eq. (3) in PRL 102, 226401 (2009)] is calculated.
>
>                               According to a test that I've just made it does not matter which one
>                               of these two is specified in case.in0_grr:
>                               "EX_GRR EC_NONE VX_GRR VC_NONE"
>                               "EX_GRR VX_GRR"
>
>                               So, I don't understand why you got two different results.
>                               Can you show us the input files case.in0 and case.in0_grr
>                               that you used for the two calculations?
>
>                               F. Tran
>
>                               On Mon, 14 Dec 2015, shima pourrad wrote:
> 
>
>                                     Dear P.Blaha and F.Tran and Wien2k Users
>
>                                     I am running wien version14.2 .The purpose of my calculations is to get accurate gap and band
>                         structure. Hence I am performing MBJ calculations with the parameters special to semiconductors.
>
>                                     I would like to ask how we should edit case.in0_grr for a mbj calculation in wien2k14.2 ?
>
>                                     I read the user guide and checked the mailing list before, I didn’t find any obvious
>                         instruction.
>
>                                     In user guide, it was written that: when you perform init_mbj_lapw for the second time, some
>                         steps must do automatically:
>
>                                      *
>                                         edit case.in0 and change the functional to option XC_MBJ. (ok this step is done).
>
>                                      *
>                                          cp case.in0 case.in0_grr and choose EX_GRR VX_GRR in case.in0_grr.
>
>                                     But this step, when I open the case.in0_grr to check that, at first line, it was written that:
>                         EX_GRR EC_NONE VX_GRR VC_NONE. Is it a correct edition? Should I remove “EC_NONE VC_NONE” from the first
>                         line?
>
>                                     I think “EX_GRR EC_NONE VX_GRR VC_NONE” means that correlation energy and potential are
>                         ignored! But “EX_GRR VX_GRR” alone, means there is a kind of correlation energy and potential as a default
>                         for usual mbj calculation. Did I realize
>                                     correctly??
>
>                                     You answered the question about the use of the PBE instead of LDA for the energy before:
>                         http://www.mail-archive.com/wien%40zeus.theochem.tuwien.ac.at/msg13395.html
>
>                                     And it is stated that how we must change case.in0 .
>
>                                     But there is no instruction for case.in0_grr. What should be done for this issue?
>
>                                     (What kind of edition is correct for case.in0_grr? “EX_GRR VX_GRR”? Or “ EX_GRR EC_NONE VX_GRR
>                         VC_NONE”?? I performed both of them for one structure, and got very different result: different Gaps,
>                         different total energies and different
>                                     Fermi-energies!!! )
>
>                                     Please help me.
>
>                                     Sincerely
>
>                                     Shima M.Pourrad
>
>                                     PhD student of physics in condensed matter
>
>                                     Science and Research Branch
>                                     Islamic Azad University
> 
>
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> 
> 
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