[Wien] something about the density matrix

Peter Blaha pblaha at theochem.tuwien.ac.at
Thu Jan 30 14:33:33 CET 2020


You can check the "update" page for a history and the main changes. I'm 
quite sure that the 2016 dmat in lapw2 was not correct in all cases 
(symmetries).


On 1/30/20 1:54 PM, 姜若诗 wrote:
> I used version: WIEN2k_16.1, We don’t update the most recent version. 
> Maybe it’s something cause it wrong.
> 
> I will use WIEN2k_19.1 to do the same thing, If I still have problem, I 
> will let you know.
> 
> Thank you very much!
> 
> Regards,
> 
> Jasmine.
> 
> *From: *Peter Blaha <mailto:pblaha at theochem.tuwien.ac.at>
> *Sent: *Thursday, January 30, 2020 8:28 PM
> *To: *wien at zeus.theochem.tuwien.ac.at 
> <mailto:wien at zeus.theochem.tuwien.ac.at>
> *Subject: *Re: [Wien] something about the density matrix
> 
> Are you using the most recent WIEN2k_19.1 version ?? (Previous versions
> 
> could have had some bug).
> 
> If yes, Please send me the struct file (to my private email) and I'll
> 
> try to verify (and fix) the problem.
> 
> Regards
> 
> Peter Blaha
> 
> On 1/30/20 1:16 PM, 姜若诗 wrote:
> 
>  > Yes, everything is right, but the answer is wrong.
> 
>  >
> 
>  > However, I try to use x lapwdm to create the new density matrix, the
> 
>  > answer is different with the former density matrix which calculate by x
> 
>  > lapw2. And the new trace of density matrix is agree with the partial
> 
>  > charges sphere d orbital. ( equal to 4.24).
> 
>  >
> 
>  > Do you know why the results are different from x lapwdm and x lapw2?
> 
>  > Cause usually we don’t run the x lapwdm, we just use runsp_lapw to do
> 
>  > the calculation and the result of case.scf is from case.dmatup using x
> 
>  > lapw2, which is totally wrong. So I want to know the reason.
> 
>  >
> 
>  > Looking forward to your reply.
> 
>  >
> 
>  > Regards,
> 
>  >
> 
>  > Jasmine.
> 
>  >
> 
>  > --------------------------------------------case.dmatup  by using ‘x
> 
>  > lapwdm’------------------------------------------------
> 
>  >
> 
>  >      1 atom density matrix
> 
>  >
> 
>  >      2 -0.000000 -0.000000  0.000000 L, Lx,Ly,Lz in global orthogonal 
> system
> 
>  >
> 
>  >    8.434407350603E-01 -5.421011859548E-20   -5.767192279293E-13
> 
>  > 2.115942936830E-10
> 
>  >
> 
>  >    4.595643053517E-02 -5.186184711430E-12    2.124411757620E-12
> 
>  > 2.386160098194E-10
> 
>  >
> 
>  > -3.820409375453E-02  1.467943531265E-11
> 
>  >
> 
>  > -5.766775945659E-13 -2.115942936830E-10 8.420614513118E-01
> 
>  > 4.417621069238E-28
> 
>  >
> 
>  > -2.035371871045E-12 -5.005882217579E-10   -4.558281203922E-02
> 
>  > -1.478855820594E-12
> 
>  >
> 
>  > -2.124425635408E-12 -2.386159958874E-10
> 
>  >
> 
>  >    4.595643053517E-02  5.186184711430E-12   -2.035427382197E-12
> 
>  > 5.005882217579E-10
> 
>  >
> 
>  >    8.704389870434E-01 1.458114115773E-26    2.035427382197E-12
> 
>  > 5.005882217579E-10
> 
>  >
> 
>  >    4.595643053517E-02 -5.186184711430E-12
> 
>  >
> 
>  >    2.124439513196E-12 -2.386159958874E-10   -4.558281203922E-02
> 
>  > 1.478855820594E-12
> 
>  >
> 
>  >    2.035371871045E-12 -5.005882217579E-10 8.420614513118E-01
> 
>  > -8.456588903969E-28
> 
>  >
> 
>  >    5.766359612025E-13 -2.115942936830E-10
> 
>  >
> 
>  > -3.820409375453E-02 -1.467943531265E-11   -2.124397879832E-12
> 
>  > 2.386160098194E-10
> 
>  >
> 
>  >    4.595643053517E-02  5.186184711430E-12    5.766775945659E-13
> 
>  > 2.115942936830E-10
> 
>  >
> 
>  >    8.434407350603E-01 5.421012500103E-20
> 
>  >
> 
>  > ----------------------------------------------case.dmatup by using
> 
>  > ‘runsp_lapw’----------------------------------------------------
> 
>  >
> 
>  >      1 atom density matrix
> 
>  >
> 
>  >      2  0.000000  0.000000  0.000000 L, Lx,Ly,Lz in global orthogonal 
> system
> 
>  >
> 
>  >       2.8005160871445E-01 0.0000000000000E+00
> 
>  > -3.0216407857826E-12     6.7145677128848E-13
> 
>  >
> 
>  >       1.5324160056603E-02    -3.9664653479197E-06
> 
>  > 2.6399668898113E-12     2.0249072052783E-13
> 
>  >
> 
>  >      -1.2540961586142E-02    -9.2618304124408E-13
> 
>  >
> 
>  >      -3.0216347173528E-12    -6.7145422790243E-13 2.7994357617885E-01
> 
>  > 0.0000000000000E+00
> 
>  >
> 
>  >       2.3155181089256E-12    -8.5717374930559E-13
> 
>  > -1.5018560016544E-02     8.0191364535328E-13
> 
>  >
> 
>  >      -2.6399626062138E-12     1.6438865579330E-13
> 
>  >
> 
>  >       1.5324160056603E-02     3.9664653479197E-06
> 
>  > 2.3155163240933E-12     8.5717374930559E-13
> 
>  >
> 
>  > 2.8889820760347E-01 0.0000000000000E+00      -2.3155152531939E-12
> 
>  > -7.7723949878888E-13
> 
>  >
> 
>  >       1.5324160056603E-02     3.9664638506938E-06
> 
>  >
> 
>  >       2.6399593935156E-12    -2.0249183604803E-13
> 
>  > -1.5018560016544E-02    -8.0192060619930E-13
> 
>  >
> 
>  >      -2.3155093632472E-12     7.7723949878888E-13 2.7994357617885E-01
> 
>  > 0.0000000000000E+00
> 
>  >
> 
>  >       3.0216343603863E-12     6.3767083267023E-13
> 
>  >
> 
>  >      -1.2540961586142E-02     9.2618893119071E-13
> 
>  > -2.6399699240262E-12    -1.6439066372965E-13
> 
>  >
> 
>  >       1.5324160056603E-02    -3.9664638506938E-06
> 
>  > 3.0216479251119E-12    -6.3766699528076E-13
> 
>  >
> 
>  > 2.8005160871445E-01 0.0000000000000E+00
> 
>  >
> 
>  > 
> -------------------------------------------------------------------------------------------------------------------------------------------------
> 
>  >
> 
>  > *From: *Tran, Fabien <mailto:fabien.tran at tuwien.ac.at>
> 
>  > *Sent: *Thursday, January 30, 2020 6:39 PM
> 
>  > *To: *A Mailing list for WIEN2k users
> 
>  > <mailto:wien at zeus.theochem.tuwien.ac.at>
> 
>  > *Subject: *Re: [Wien] something about the density matrix
> 
>  >
> 
>  > In principle they should agree. Is this block of the density matrix
> 
>  > really corresponding to atom 1 and the corresponding spin?
> 
>  >
> 
>  > *From:*Wien <wien-bounces at zeus.theochem.tuwien.ac.at> on behalf of 姜若
> 
>  > 诗<ruoshijiang at sjtu.edu.cn>
> 
>  > *Sent:* Thursday, January 30, 2020 11:23 AM
> 
>  > *To:* wien at zeus.theochem.tuwien.ac.at
> 
>  > *Subject:* [Wien] something about the density matrix
> 
>  >
> 
>  > Dear all,
> 
>  >
> 
>  > I have a question, below is the data of case.scf.
> 
>  >
> 
>  > Why the trace of the density matrix is not consistent with the :QTL001,
> 
>  > partial charges sphere of the d orbital(L = 2)? Did something wrong?
> 
>  >
> 
>  > Looking forward to your reply. Thank you.
> 
>  >
> 
>  > Regards,
> 
>  >
> 
>  > Jasmine
> 
>  >
> 
>  > 
> -------------------------------------------------------------------------------------------------------------------------------------------
> 
>  >
> 
>  > :POS001: ATOM   -1 X,Y,Z = 0.75000 0.75000 0.50000  MULT= 4  ZZ= 
> 28.000  Ni1
> 
>  >
> 
>  >         LMMAX 16
> 
>  >
> 
>  >         LM=   0 0  1 0  2 0  2 2  3 0  3 2  4 0  4 2  4 4  5 0  5 2  5
> 
>  > 4  6 0  6 2  6 4  6 6
> 
>  >
> 
>  > :CHA001: TOTAL VALENCE CHARGE INSIDE SPHERE   1 =   7.4660    (RMT=
> 
>  > 1.9800 )
> 
>  >
> 
>  > :PCS001: PARTIAL CHARGES SPHERE =  1
> 
>  > S,P,D,F,PX,PY,PZ,D-Z2,D-X2Y2,D-XY,D-XZ,D-YZ
> 
>  >
> 
>  > :QTL001: 0.1192 3.0914 4.2412 0.0112 1.0134 1.0390 1.0389 0.8706 0.8050
> 
>  > 0.8816 0.8877 0.7962
> 
>  >
> 
>  >          Q-s-low E-s-low   Q-p-low E-p-low   Q-d-low E-d-low   Q-f-low
> 
>  > E-f-low
> 
>  >
> 
>  > :EPL001:  0.0137 -0.7431    3.0018 -4.1369    0.0179 -0.6935    0.0022
> 
>  > -0.7084
> 
>  >
> 
>  >          Q-s-hi  E-s-hi    Q-p-hi  E-p-hi    Q-d-hi  E-d-hi    Q-f-hi
> 
>  > E-f-hi
> 
>  >
> 
>  > :EPH001:  0.1054  0.2634    0.0897  0.2885    4.2235  0.4988    0.0092
> 
>  > 0.3393
> 
>  >
> 
>  > Density matrix      block, real part.  L= 2
> 
>  >
> 
>  > 0.28001 0.00000  0.01533  0.00000 -0.01255
> 
>  >
> 
>  >           0.00000 0.27989 0.00000 -0.01501  0.00000
> 
>  >
> 
>  >           0.01533  0.00000 0.28883 0.00000  0.01533
> 
>  >
> 
>  >           0.00000 -0.01501  0.00000 0.27989 0.00000
> 
>  >
> 
>  >          -0.01255  0.00000  0.01533  0.00000 0.28001
> 
>  >
> 
>  > Density matrix, imag part
> 
>  >
> 
>  >           0.00000  0.00000  0.00000  0.00000  0.00000
> 
>  >
> 
>  >           0.00000  0.00000  0.00000  0.00000  0.00000
> 
>  >
> 
>  >           0.00000  0.00000  0.00000  0.00000  0.00000
> 
>  >
> 
>  >           0.00000  0.00000  0.00000  0.00000  0.00000
> 
>  >
> 
>  >           0.00000  0.00000  0.00000  0.00000  0.00000
> 
>  >
> 
>  > 
> -------------------------------------------------------------------------------------------------------------------------------------------
> 
>  >
> 
>  >
> 
>  > _______________________________________________
> 
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> 
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> 
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>  >
> 
> -- 
> 
>                                         P.Blaha
> 
> --------------------------------------------------------------------------
> 
> Peter BLAHA, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna
> 
> Phone: +43-1-58801-165300             FAX: +43-1-58801-165982
> 
> Email: blaha at theochem.tuwien.ac.at    WIEN2k: http://www.wien2k.at
> 
> WWW:   http://www.imc.tuwien.ac.at/TC_Blaha
> 
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-- 

                                       P.Blaha
--------------------------------------------------------------------------
Peter BLAHA, Inst.f. Materials Chemistry, TU Vienna, A-1060 Vienna
Phone: +43-1-58801-165300             FAX: +43-1-58801-165982
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